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Formulation of SYNROC-D additives for Savannah River Plant high-level radioactive waste. [ADSYN code]

Technical Report ·
DOI:https://doi.org/10.2172/5294246· OSTI ID:5294246
SYNROC-D is a multiphase ceramic waste form consisting of nepheline, zirconolite, perovskite, and spinel. It has been formulated for the immobilization of high-level radioactive wastes now stored at Savannah River Plant (SRP) near Aiken, South Carolina. This report utilizes existing experimental data to develop a method for calculating additives to these waste products. This method calculates additions based on variations of mineral compositions as a function of sludge composition and radionuclide partitioning among the SYNROC phases. Based on these calculations, a FORTRAN program called ADSYN has been developed to determine the proper reagent proportions to be added to the SRP sludges.
Research Organization:
Lawrence Livermore National Lab., CA (USA)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
5294246
Report Number(s):
UCRL-53237; ON: DE82012495
Country of Publication:
United States
Language:
English