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Beryllium isotope geochemistry in tropical river basins

Journal Article · · Geochimica et Cosmochimica Acta; (United States)
;  [1]; ; ;  [2];  [3]
  1. Massachusetts Inst. of Tech., Cambridge (United States)
  2. Centre National de la Recherche Scientifique, Orsay (France)
  3. Univ. of Hawaii, Honolulu (United States)

The distributions of beryllium-9 and beryllium-10 in rivers within the Orinoco and Amazon basins have been examined to extend the understanding of their geochemical cycles and to develop their use both in geochronometry, and in studying erosional processes. Analyses of {sup 9}Be in dissolved and suspended material from rivers with a wide range of chemical compositions indicate that its geochemistry is primarily controlled by two major factors: (1) its abundance in the rocks of the watershed and (2) the extent of its adsorption onto particle surfaces. The relative importance of these parameters in individual rivers is determined by the extent of interaction with flood-plain sediments and the riverine pH. This understanding of {sup 9}Be geochemistry forms a basis for examination of the geochemical cycling of {sup 10}Be. In rivers which are dominated by interaction with sediments, the riverine concentration of dissolved {sup 10}Be is far lower than that in the incoming rainwater, indicating that a substantial proportion of it is retained within the soils of the basin or is adsorbed onto riverine particles. However, in acidic rivers in which the stable dissolved Be concentration is determined by the Be level in the rocks of the drainage basin, dissolved {sup 10}Be has essentially the same concentration as in precipitation. These observations imply that the soil column in such regions must be saturated with respect to {sup 10}Be, and that the ratio of the inventory to the flux does not represent an age, as may be the case in temperate latitudes, but rather a residence time.

OSTI ID:
5262849
Journal Information:
Geochimica et Cosmochimica Acta; (United States), Journal Name: Geochimica et Cosmochimica Acta; (United States) Vol. 56:4; ISSN GCACA; ISSN 0016-7037
Country of Publication:
United States
Language:
English