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Fracture mechanisms in monolithic structural ceramics and ceramic composites

Thesis/Dissertation ·
OSTI ID:5247268

The fracture of three structurally distinct materials was characterized at test temperatures ranging from 20 through 1400{degree}C. Two monolithic, polycrystalline ceramic materials, one a high-purity transparent MgAl{sub 2}O{sub 4} spinel and the other a sintered Si{sub 3}N{sub 4} containing a grain-boundary, second-phase, sintering additive, provided for a comparison of the fracture mechanisms as they are governed by the differing microstructures. The third, a SiC whisker-reinforced, polycrystalline Al{sub 2}O{sub 3} matrix composite offered the added mechanism of a high-strength, high-modulus load-carrying element, not available in conventional, monolithic ceramic microstructures. The high-purity MgAl{sub 2}O{sub 4} spinel was found to maintain a constant fracture toughness of approximately 1.7 MPa{center dot}m{sup {1/2}} through 600{degree}C and then experienced only a slight decrease above this temperature to about 1.3 MPa{center dot}{sup {1/2}}. By comparison, the fracture toughness of the Si{sub 3}N{sub 4} decreased from nearly 8.0 MPa{center dot}m{sup {1/2}} at room temperature, to below 2.0 MPa{center dot}{sup {1/2}} 1400{degree}C, as governed by the character of the grain boundary glass phase. The SiC whisker/Al{sub 2}O{sub 3} composite was characterized by a fracture toughness value of about 6.8 MPa{center dot}{sup 1/2} throughout the test temperature range.

Research Organization:
Washington Univ., Seattle, WA (USA)
OSTI ID:
5247268
Country of Publication:
United States
Language:
English