Mass-transfer-limited release of a soluble waste species
Conference
·
· Trans. Am. Nucl. Soc.; (United States)
OSTI ID:5194602
The authors have earlier presented analytical solutions for the rates of dissolution of solubility-limited species from solid waste imbedded in saturated porous rock. The dissolution rate of some species, however, may not be limited by solubility of the species or of the waste matrix. For example, the portion of the fission product cesium and iodine in spent fuel that exists in the fuel/cladding gap and in voids and grain boundaries is available for rapid dissolution if exposed to ground water. Even though dissolution may be rapid, the rate of release of these soluble species from the waste package will be limited by the rate of mass transfer of the dissolved species through the surrounding porous media. Here the authors present the results of a new mass transfer analysis of the time-dependent release rate of species that can dissolve rapidly from the gap activity and more slowly from the waste matrix, as limited by molecular diffusion into surrounding porous rock.
- Research Organization:
- Univ. of California, Berkeley (USA)
- OSTI ID:
- 5194602
- Report Number(s):
- CONF-860610-Summs.
- Conference Information:
- Journal Name: Trans. Am. Nucl. Soc.; (United States) Journal Volume: 52
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
052002* -- Nuclear Fuels-- Waste Disposal & Storage
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
ALKALI METALS
CESIUM
ELEMENTS
ENERGY SOURCES
ENVIRONMENTAL TRANSPORT
FISSION PRODUCTS
FUELS
GROUND WATER
HALOGENS
HIGH-LEVEL RADIOACTIVE WASTES
HYDROGEN COMPOUNDS
IODINE
ISOTOPES
MANAGEMENT
MASS TRANSFER
MATERIALS
METALS
NONMETALS
NUCLEAR FUELS
OXYGEN COMPOUNDS
RADIOACTIVE MATERIALS
RADIOACTIVE WASTES
RADIONUCLIDE MIGRATION
REACTOR MATERIALS
SOLUBILITY
SPENT FUELS
TIME DEPENDENCE
UNDERGROUND DISPOSAL
WASTE DISPOSAL
WASTE MANAGEMENT
WASTES
WATER
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
ALKALI METALS
CESIUM
ELEMENTS
ENERGY SOURCES
ENVIRONMENTAL TRANSPORT
FISSION PRODUCTS
FUELS
GROUND WATER
HALOGENS
HIGH-LEVEL RADIOACTIVE WASTES
HYDROGEN COMPOUNDS
IODINE
ISOTOPES
MANAGEMENT
MASS TRANSFER
MATERIALS
METALS
NONMETALS
NUCLEAR FUELS
OXYGEN COMPOUNDS
RADIOACTIVE MATERIALS
RADIOACTIVE WASTES
RADIONUCLIDE MIGRATION
REACTOR MATERIALS
SOLUBILITY
SPENT FUELS
TIME DEPENDENCE
UNDERGROUND DISPOSAL
WASTE DISPOSAL
WASTE MANAGEMENT
WASTES
WATER