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Selective counting of krypton atoms using resonance ionization spectroscopy

Journal Article · · Appl. Phys. Lett.; (United States)
DOI:https://doi.org/10.1063/1.94861· OSTI ID:5178681
Resonance ionization spectroscopy (RIS) was used to count 1000 individual /sup 81/Kr atoms. In the method, lasers for RIS are used to obtain atomic species (Z) selectivity and a small quadrupole mass spectrometer provides isotopic (A) selectivity. After Z and A selection the krypton ions were counted as they were implanted into a target. Basically, the method works for any isotope whether stable or unstable. However, the detection limit may depend on the isotope because of outgassing of stable atoms from the enclosure walls. For /sup 81/Kr, we show that fewer than 1000 atoms can be counted with good accuracy.
Research Organization:
Chemical Physics Section, Health and Safety Research Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
DOE Contract Number:
W-7405-ENG-26
OSTI ID:
5178681
Journal Information:
Appl. Phys. Lett.; (United States), Journal Name: Appl. Phys. Lett.; (United States) Vol. 44:6; ISSN APPLA
Country of Publication:
United States
Language:
English