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Sol-gel synthesis of protoenstatite

Book ·
OSTI ID:51595
;  [1]
  1. Cornell Univ., Ithaca, NY (United States). Dept. of Chemistry

Protoenstatite, a high-temperature polymorph of enstatite (MgSiO{sub 3}), is generally not stable at room temperature, and is difficult to synthesize. Using a recently developed, hydrogen peroxide assisted, sol-gel synthesis, protoenstatite was synthesized in a form that was stable at room temperature. Its crystallization was strongly dependent on processing conditions, particularly on the manner in which the xerogel was formed and fired. Xerogels prepared by evaporation, spray-drying and freeze-drying were compared by XRD, HTXRD, BET, TG/DTA, and {sup 29}Si NMR methods. When samples were prepared by evaporation or spray-drying, the result was a mixture of polymorphs. Only the freeze-dried precursor yielded protoenstatite at a lower temperature and within a shorter time than any previously reported.

OSTI ID:
51595
Report Number(s):
CONF-940411--; ISBN 1-55899-246-4
Country of Publication:
United States
Language:
English

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