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U.S. Department of Energy
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Technetium-99 in the atmosphere

Journal Article · · Environ. Sci. Technol.; (United States)
DOI:https://doi.org/10.1021/es60137a006· OSTI ID:5116503
The technetium 99 and strontium 90 concentrations were measured from a composite rain sample (1015 L) collected in the spring of 1975. The concentrations were (4.5 +- 1.5) x 10/sup -3/ and 0.11 +- 0.02 dpm/L, respectively. The results indicated that /sup 99/Tc concentration decreased from those samples measured in 1961, 1962, and 1967, whereas the /sup 99/Tc//sup 90/Sr ratio showed a steady increase during this time period. All observed /sup 99/Tc//sup 90/Sr values were larger than the anticipated values from the neutron-induced fission of /sup 235/U or /sup 239/Pu, indicating sources of /sup 99/Tc other than fission.
Research Organization:
East Texas State Univ., Commerce
OSTI ID:
5116503
Journal Information:
Environ. Sci. Technol.; (United States), Journal Name: Environ. Sci. Technol.; (United States) Vol. 12:1; ISSN ESTHA
Country of Publication:
United States
Language:
English