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Transport and magnetic properties of icosahedral and glassy Pd-U-Si alloys

Journal Article · · Phys. Rev. B: Condens. Matter; (United States)

The glassy phase of Pd/sub 58.8/U/sub 20.6/Si/sub 20.6/ alloys can be transformed into an icosahedral quasicrystalline phase by thermal annealing. Electrical transport properties of samples undergoing different degrees of glassy-to-icosahedral phase transformation have been measured. The icosahedral phase has an electrical resistivity of --220 ..mu cap omega.. cm at room temperature and a negative temperature coefficient of resistivity. The short electronic mean free path is discussed. At low temperature, the negative magnetoresistivity is attributed to magnetic scattering effects. The low-field ac susceptibility as a function of temperature exhibits a spin-glass-type transition which is not suppressed by a dc magnetic field.

Research Organization:
Department of Physics, University of Virginia, Charlottesville, Virginia 22901
OSTI ID:
5113558
Journal Information:
Phys. Rev. B: Condens. Matter; (United States), Journal Name: Phys. Rev. B: Condens. Matter; (United States) Vol. 34:10; ISSN PRBMD
Country of Publication:
United States
Language:
English