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Isothermal diffusion coefficients for NaCl-MgCl sub 2 -H sub 2 O at 25 degree C. 1. Solute concentration ratio of 3:1

Journal Article · · Journal of Physical Chemistry; (USA)
DOI:https://doi.org/10.1021/j100342a090· OSTI ID:5093546
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  1. Lawrence Livermore National Lab., CA (USA)

Isothermal interdiffusion coefficients have been obtained by Gouy interferometry for the ternary system NaCl-MgCl{sub 2}-H{sub 2}O at 25.00{degree}C and at a 3:l molarity ratio of NaCl to MgCl{sub 2}. Data are reported for total molar concentrations of 0.5, 1 .0, 2.0, 3.0, and 3.79 M. One cross-term diffusion coefficient, D{sub 12}, becomes greater than all the other diffusion coefficients above 3.2 M. This shows that at higher concentrations a flow of NaCl resulting from a concentration gradient of MgCl{sub 2} will be greater than the flow resulting from the same concentration gradient of NaCl itself. Also, a concentration gradient of MgCl{sub 2} will cause a greater flow of NaCl than of MgCl{sub 2} itself. Densities were measured for all the solutions; they were used to calculate partial-molal volumes of all components in the solutions and to interconvert reference frames for diffusion.

DOE Contract Number:
W-7405-ENG-48
OSTI ID:
5093546
Journal Information:
Journal of Physical Chemistry; (USA), Journal Name: Journal of Physical Chemistry; (USA) Vol. 93:5; ISSN 0022-3654; ISSN JPCHA
Country of Publication:
United States
Language:
English