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Concentrations of uranium and thorium isotopes in uranium millers' and miners' tissues

Technical Report ·
OSTI ID:5090285

The alpha-emitting isotopes of uranium and thorium were determined in the lungs of 14 former uranium miners and in soft tissues and bones of three miners and two millers. These radionuclides were also determined in soft tissues and bones of seven normal controls. The average concentrations in pCi/kg wet weight in 17 former miners' lungs are as follows: /sup 238/U, 75; /sup 234/U, 80; /sup 230/Th, 79. Concentrations of each nuclide ranged from 2 to 325 pCi/kg. The average ratio of /sup 238/U//sup 234/U was 0.92, ranging from 0.64 to 1.06. The mean ratio of /sup 230/Th//sup 234/U was 1.04, ranging from 0.33 to 3.54. The near equilibrium between /sup 230/Th and /sup 238,234/U indicates that the rate of elimination of uranium and thorium from lungs is the same in former uranium miners. The concentrations of /sup 234/U and /sup 238/U were highest in lung; however, the concentration of /sup 230/Th in bones was either higher than or comparable to its concentration in lung. The concentration ratios of /sup 230/Th//sup 234/U in bone of uranium miners and millers measured in our laboratory have been compared with results predicted by ICRP-30 metabolic models. These results indicate that the ICRP metabolic models for thorium and uranium were only marginally successful in predicting the ratio of /sup 230/Th//sup 234/U in bones, and that effective release rate of uranium from skeleton may be more rapid than predicted by the ICRP model. 9 figs., 21 tabs.

Research Organization:
Utah Univ., Salt Lake City (USA). Radiobiology Lab.
OSTI ID:
5090285
Report Number(s):
NUREG/CR-4382; ON: TI86900088
Country of Publication:
United States
Language:
English