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Title: Impact of urban and industrial emissions on mesoscale precipitation quality

Journal Article · · J. Air Pollut. Control Assoc.; (United States)

Results from an acid rain field study around the city of Philadelphia are presented. The study involved the sampling of wet deposition at a network of 40 sites within a distance of 60 km from the Delaware River. Emphasis was placed on event-type rain sampling of frontal and primarily nonconvective storms which are responsible for most of the Northeast's wet deposition. For most storms, meteorological conditions contributed to a predominant southeasterly transport. Local emissions appear to impact the deposition of nitrate (NO/sub 3//sup -/ which may register increases greater than 200%. It appears that this impact grows with distance from the river suggesting peaks beyond the 60 km boundary of the network. Comparisons with estimates of NO/sub x/ emissions reveal that a substantial fraction may be deposited as NO/sub 3//sup -/ on the mesoscale. The impact of local emissions on total sulfur is less striking; for some storms the sulfur excess is only in the form of dissolved SO/sub 2/.

Research Organization:
Brookhaven National Lab. (BNL), Upton, NY (United States)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
5027627
Journal Information:
J. Air Pollut. Control Assoc.; (United States), Vol. 35:7
Country of Publication:
United States
Language:
English