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Fission Product Release from Overheated Uranium - A Laboratory Study

Journal Article · · Health Physics

Preliminary tests investigated the oxidation and ignition behavior of unirradiated uranium in air and steam. Small uranium cylinders were then irradiated to 2 x 1014 nvt and heated out-of-reactor under carefully controlled conditions, and the fractions of the fission product isotopes leaving the specimen were determined. Temperatures up to 1440 deg C for as long as 4 hr in atmospheres of air, steam, and helium were measured; release in air was from two to ten times greater than in steam, while in helium the release was v'ery low. Iodine, tellurium, and xenon were released in proportion to the amount of uranium oxidized. Cesium and ruthenium were found to be semi-volatile. The release of strontium, barium, and zirconium was found to be less than 0.2% under all conditions tested. Efiiciencies of several filter media in retaining volatilized fission products were also measured.

Research Organization:
General Electric Co., Richland, Wash.
Sponsoring Organization:
USDOE
NSA Number:
NSA-16-009047
OSTI ID:
4808403
Report Number(s):
HW-SA-2040; 0017-9078
Journal Information:
Health Physics, Journal Name: Health Physics Journal Issue: 1 Vol. 7; ISSN 0017-9078
Publisher:
Health Physics Society
Country of Publication:
Country unknown/Code not available
Language:
English