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Multielectron Dissociative Ionization of Molecules by Intense Laser Radiation

Journal Article · · Physical Review Letters
 [1];  [2];  [3]
  1. Filia Uniwersytetu Warszawskiego, ul.Lipowa 41, 15-424 Bialystok (Poland)
  2. Centrum Fizyki Teoretycznej PAN and College of Science, Al.Lotnikow32/46, 02-668 Warsaw (Poland)
  3. Electron and Optical Physics Division, Physics Laboratory, National Institute of Standards and Technology, Technology Administration, U.S. Department of Commerce, Gaithersburg, Maryland 20899 (United States)
We solve the hydrodynamic-ballistic equations of motion for a one-dimensional time-dependent Thomas-Fermi model of Cl{sub 2} exposed to an intense subpicosecond laser field, and observe simultaneous multielectron ionization and molecular dissociation. The fragment kinetic energy defect with respect to the simple Coulomb explosion picture is found to originate in ejected-electron screening of the escaping fragments; its magnitude agrees with that observed in recent experiments.
OSTI ID:
471194
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 2 Vol. 78; ISSN 0031-9007; ISSN PRLTAO
Country of Publication:
United States
Language:
English

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