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Synergistic solvent extraction of trivalent lanthanides with mixtures of 3-phenyl-4-benzoyl-5-isoxazolone and crown ethers

Journal Article · · Solvent Extraction and Ion Exchange

Synergistic solvent extraction of trivalent lanthanides such as Nd, Eu and Tm has been studied using mixtures of 3-phenyl-4-benzoyl-5-isoxazolone (HPBI) and 18-crown-6, 15-crown-5, benzo-15-crown-5, or dibenzo-18-crown-6. The results demonstrate that these trivalent metal ions are extracted into chloroform as Ln(PBI){sub 3} with HPBI alone and as Ln(PBI){sub 3}. CE in the presence of crown ethers (CE). The equilibrium constants of the above species are found to increase monotonically with the decreasing ionic radii of these trivalent lanthanides. The addition of a crown ether to the metal chelate system significantly enhances the extractability of these trivalent metal ions. 23 refs., 3 figs., 4 tabs.

Sponsoring Organization:
USDOE
OSTI ID:
466331
Journal Information:
Solvent Extraction and Ion Exchange, Journal Name: Solvent Extraction and Ion Exchange Journal Issue: 1 Vol. 15; ISSN 0736-6299; ISSN SEIEDB
Country of Publication:
United States
Language:
English

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