The source identification of ambient aerosols in Beijing, China by multivariate analysis coupled with {sup 14}C tracer
- Peking Univ., Beijing (China)
Ambient aerosol is one of most important pollutants in China. This paper showed the results of aerosol sources of Beijing area revealed by combination of multivariate analysis models and 14C tracer measured on Accelerator Mass Spectrometry (AMS). The results indicated that the mass concentration of particulate (<100 (M)) didn`t increase rapidly, compared with economic development in Beijing city. The multivariate analysis showed that the predominant source was soil dust which contributed more than 50% to atmospheric particles. However, it would be a risk to conclude that the aerosol pollution from anthropogenic sources was less important in Beijing city based on above phenomenon. Due to lack of reliable tracers, it was very hard to distinguish coal burning from soil source. Thus, it was suspected that the soil source above might be the mixture of soil dust and coal burning. The 14C measurement showed that carbonaceous species of aerosol had quite different emission sources. For carbonaceous aerosols in Beijing, the contribution from fossil fuel to ambient particles was nearly 2/3, as the man-made activities ( coal-burning, etc.) increased, the fossil part would contribute more to atmospheric carbonaceous particles. For example, in downtown Beijing at space-heating seasons, the fossil fuel even contributed more than 95% to carbonaceous particles, which would be potential harmful to population. By using multivariate analysis together with 14C data, two important sources of aerosols in Beijing (soil and coal) combustion were more reliably distinguished, which was critical important for the assessment of aerosol problem in China.
- OSTI ID:
- 466184
- Report Number(s):
- CONF-9606185-; TRN: 96:005931-0135
- Resource Relation:
- Conference: 5. international conference on atmospheric sciences and applications to air quality, Seattle, WA (United States), 18-20 Jun 1996; Other Information: PBD: 1996; Related Information: Is Part Of The 5th international atmospheric sciences and applications to air quality conference; PB: 322 p.
- Country of Publication:
- United States
- Language:
- English
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