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High-intensity laser heating in liquids: Multiphoton absorption

Book ·
OSTI ID:462592
;  [1]
  1. Univ. of California, Berkeley, CA (United States). Dept. of Mechanical Engineering

At high laser intensities, otherwise transparent liquids can absorb strongly by the mechanism of multiphoton absorption, resulting in absorption and heating several orders of magnitude greater than classical, low-intensity mechanisms. The use of multiphoton absorption provides a new mechanism for strong, controlled energy deposition in liquids without bulk plasma formation, shock waves, liquid ejection, etc., which is of interest for many laser-liquid applications, including laser desorption of liquid films, laser particle removal, and laser water removal from microdevices. This work develops a microscopically based model of the heating during multiphoton absorption in liquids. The dependence on pulse duration, intensity, wavelength, repetition rate, and liquid properties is discussed. Pure water exposed to 266 nm laser radiation is investigated, and a novel heating mechanism for water is proposed that uses multiple-wavelength laser pulses.

Sponsoring Organization:
USDOE, Washington, DC (United States); National Science Foundation, Washington, DC (United States)
OSTI ID:
462592
Report Number(s):
CONF-950828--; ISBN 0-7918-1705-9
Country of Publication:
United States
Language:
English

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