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Modeling of gaseous flows within proton exchange membrane fuel cells

Technical Report ·
DOI:https://doi.org/10.2172/460311· OSTI ID:460311
;  [1];  [2]
  1. Los Alamos National Lab., NM (United States)
  2. Delphi Energy and Engine Management Systems, Rochester, NY (United States)

Development of a comprehensive mechanistic model has been helpful to understand PEM fuel cell performance. Both through-the-electrode and down-the-channel models have been developed to support our experimental effort to enhance fuel cell design and operation. The through-the-electrode model was described previously. This code describes the known transport properties and dynamic processes that occur within a membrane and electrode assembly. Key parameters include transport through the backing layers, water diffusion and electroosmotic transport in the membrane, and reaction electrochemical kinetics within the cathode catalyst layer. In addition, two geometric regions within the cathode layer are represented, the first region below saturation and second with liquid water present. Although processes at high gas stoichiometry are well represented by more simple codes, moderate stoichiometry processes require a two dimensional representation that include the gaseous composition and temperature along flow channel. Although usually PEM hardware utilizes serpentine flow channels, this code does not include such geometric features and thus the flow can be visualized along a single channel.

Research Organization:
Fuel Cell Seminar Organizing Committee (United States)
DOE Contract Number:
AC02-90CH10435
OSTI ID:
460311
Report Number(s):
CONF-961107--Absts.; ON: TI97001494
Country of Publication:
United States
Language:
English

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