Fine mode aerosol composition at three long-term atmospheric monitoring sites in the Amazon Basin
- Universidade de Sao Paulo, Sao Paulo (Brazil)
The Amazon Basin tropical rain forest is a key region to study processes that are changing the composition of the global atmosphere, including the large amount of fine mode aerosol particles emitted during biomass burning that might influence the global atmosphere. Three background monitoring stations, Alta Floresta, Cuiaba, and Serra do Navio, are operating continuously measuring aerosol composition. Fine (particle diameter less than 2.0 microns) and coarse (particle diameter greater than 2.0 microns and less than 10 microns) mode aerosol particles were collected using stacked filter units. Particle-induced X-ray emission was used to measure concentrations of up to 20 elements in the fine mode: Al, Si, P, S, Cl, K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, Br, Rb, Sr, Zr, and Pb. Soot carbon and gravimetric mass analysis were also performed. Absolute Principal Factor Analysis (APFA) has derived absolute elemental source profiles. APFA showed four aerosol particle components: soil dust (Al, Ca, Ti, Mn, Fe), biomass burning (soot, fine mode mass concentration, K, Cl), natural primary biogenic particles with gas-to-particle component (K, S, Ca, Mn, Zn), and marine aerosol (Cl). Biogenic and biomass burning aerosol particles dominate the fine mode mass concentration, with the presence of K, P, S, Cl, Zn, Br, and fine mode mass concentration (FPM). At the Alta Floresta and Cuiaba sites, during the dry season, a strong component of biomass burning is observed. Inhalable particulate matter (particle diameter less than 10 microns) mass concentration up to 700 micrograms/cu m was measured. Fine particle mass concentration alone can go as high as 400 micrograms/cu m for large regions.
- Sponsoring Organization:
- USDOE
- OSTI ID:
- 45814
- Journal Information:
- Journal of Geophysical Research, Journal Name: Journal of Geophysical Research Journal Issue: D11 Vol. 99; ISSN JGREA2; ISSN 0148-0227
- Country of Publication:
- United States
- Language:
- English
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