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NEPTUNIUM ISOTOPES: 234, 235, 236

Journal Article · · Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D
Neptunium isotopes of mass numbers 234, 235, and 236 were produced by an 18-Mev deuteron bombardment of uranium highly enriched in U/sup 235/. The radiations of Np/sup 235/ were studied with scintillation and proportional counters in singles and coincidence. The L/K and M/L electron capture branching ratios of Np/sup 235/ were measured to be 36.7 and 0.46, respectively. From the L/K ratio, the calculated decay energy of Np/sup 235/ is 123 kev. An upper limit of 2.1% of the Np/sup 235/ electron capture disintegrations populate excited states of U/sup 235/. The experimental data favor a spin of 5/2 for Np/sup 235/. The alpha to electron capture ratio for Np/sup 235/ is 1.59 x 10/sup -5/, giving a partial alpha halflife of 7.0 x 10/sup 4/ years. The long-lived isomer of Np/ sup 236/ was produced in the bombardment, but no isomer of Np/sup 234/ with half-life longer than two months was observed in a mass spectrometer analysis of the neptunium sample. (auth)
Research Organization:
Argonne National Lab., Lemont, Ill.
NSA Number:
NSA-12-006543
OSTI ID:
4331078
Journal Information:
Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D, Journal Name: Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D Vol. Vol: 109; ISSN PHRVA
Country of Publication:
Country unknown/Code not available
Language:
English