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MASS-SPECTROMETRIC STUDIES OF PILE POISONS AND THEIR YIELDS IN THE FISSION OF U-233, U-235, AND Pu-239

Technical Report ·
OSTI ID:4264936
obtained at various neutron fluxes and irradiation times has made possible the measurement of pileneutron absorption resulting from the accumulation of several fission products in a D/sub 2/O-moderated reactor. The following pile-neutron absorption cross sections have been measured relative to Co/sup 59/ = 36.0 barns: Cs/sup 133/ = 40 barns, Pm/sup 147/ = 207 barns, Sm/sup 149/ = 85,000 barns, Sm/sup 151/ = 11,500 barns. Some of these values are considerably higher than thermal-neutron values because of resonance absorption. Cumulative yields of each of these nuclides as well as those of the 135 and 143 mass chains have also been measured by isotopedilution techniques for the thermal- neutron fission of U/sup 233/ and Pu /sup 239/. These measurements, together with the previously published cross section of Xe/sup 135/ and fission yields for U/sup 235/, make possible a comparison of these poisons in reactors using U/sup 233/, U/sup 235/, and Pu/sup 239/ fuels. In twenty-three mass chains where the stable or longlived end products have low absorption cross sections, it has been possible to eliminate the possibility of significant neutron absorption amongst the short-lived precursors. (auth)
Research Organization:
McMaster Univ., Hamilton, Ont.
NSA Number:
NSA-13-006962
OSTI ID:
4264936
Report Number(s):
A/CONF.15/P/201; AECL-611
Country of Publication:
Country unknown/Code not available
Language:
English