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SOME CHEMICAL PROBLEMS OF HOMOGENEOUS AQUEOUS REACTORS

Technical Report ·
OSTI ID:4263916
The basic chemical and energy aspects of aqueous homogeneous reactors were investigated. The primary effort was devoted to the two-one uranyl sulfate solution/thoria slurry system. Corrosion associated with the neutron window of the two-zone system is discussed, together with various methods of decreasing the rate of attack. The feasibility of the use of uranyl nitrate as the fissile solution and thorium nitrate as a fertile solution was examined. Thorium nitrate may find applications in core solutions, if the processing rate is sufficient to maintain a low uranium content. The rheology of aqueous slurries of thoria is described, and measurements in a pipe-line viscometer are compared with the result of pumping the same slurry in a loop system. Plutonium dioxide suspensions were examined for use in the fuel circuit of a burner reactor. The physical properties of the oxide prepared by various methods were measured, and electrophoretic properties were compared with those of thoria. (J.R.D.)
Research Organization:
Atomic Energy Research Establishment, Harwell, Berks, Eng. (United Kingdom)
NSA Number:
NSA-13-007083
OSTI ID:
4263916
Report Number(s):
A/CONF.15/P/46
Country of Publication:
United Kingdom
Language:
English