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THE CHEMICAL DETERMINATION OF BORON IN BORON CARBIDE-ZIRCONIUM, CLAD WITH ZIRCALOY

Technical Report ·
DOI:https://doi.org/10.2172/4263443· OSTI ID:4263443

A rapid dissolution chemical method for the determination of boron in Zircaloy-clad boron carbideolved in a tained in a platinum dish which is cooled in a dry-ice bed. Approximately 96 to 99% of the total boron remains undissolved. This is filtered off, ashed, fused with sodium carbonate, and the boron is determined according to mannitol titration method. The acidsoluble boron is determined by a modified mannitol titration after separating the zirconium and other interfering cations with barium carbonate. The acidinsoluble and acid- soluble boron are added to give the total boron in the sample. The accuracy and precision of this analysis were checked on synthetic mixtures of standard'' boron carbide plus zirconium. At the 2% boron carbide (1.59% B) level or higher, the method was accurate to at least 1.15 relative per cent. The precision (95% confidence level) was plus or minus 0.27 and plus or minus 0.95 relative per cent based on 8 measurements or a single measurement, respectively. Standardization'' of the boron carbide sample was performed by analyzing for boron, carbon, and impurities. A mass balance of 100.22 plus or minus 0.69% was obtained and the boron value waa considered accurate within the precision of the analytical method. ( auth)

Research Organization:
Knolls Atomic Power Lab., Schenectady, N.Y.
DOE Contract Number:
W-31-109-ENG-52
NSA Number:
NSA-13-017798
OSTI ID:
4263443
Report Number(s):
KAPL-M-JR-12
Country of Publication:
United States
Language:
English