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Isotopic ratios of iodine and other radionuclides as nuclear power pollution indicators

Conference ·
OSTI ID:4160280
The determination of isotope ratios in addition to radionuclide concentrations is useful in the identification and tracing of radioactive pollutant sources. Methods have been developed for measurement of $sup 58$Co/ $sup 60$Co, $sup 134$Cs/$sup 137$Cs, $sup 129$I/$sup 127$I and other radionuclide effluent isotope ratios at levels much below those required for radiation protection. Measurements of $sup 58$Co/$sup 60$Co, $sup 134$Cs/$sup 137$Cs, $sup 135$Cs/$sup 137$Cs and $sup 129$I/$sup 127$I in environmental samples have demonstrated their application to the detection of nuclear plant effluents. Increased $sup 129$I/$sup 127$I ratios were observed in nuclear fuel separations facility environs at levels much below radiation protection standards. The pathways in the transfer of atmospheric $sup 129$I to food materials has been studied by means of $sup 129$I/$sup 127$I analyses of environmental samples. Vegetation absorption of atmospheric iodine was found to be significant. The $sup 129$I/$sup 127$I ratio was observed to decrease in the pathway from the atmosphere to food. Examples of the use of $sup 129$I analysis for environmental studies are presented. (auth)
Research Organization:
Battelle-Pacific Northwest Labs., Richalnd, WA
NSA Number:
NSA-33-007287
OSTI ID:
4160280
Country of Publication:
IAEA
Language:
English