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DETERMINATION OF TETRAVALENT URANIUM IN THORIUM OXIDE-URANIUM OXIDE MIXTURES. PARTS I, II, AND III

Technical Report ·
DOI:https://doi.org/10.2172/4117883· OSTI ID:4117883

For the determination of milligram quantities of uranium(N) in thorium oxide-uranium oxide mixtures which may also contain uranium(VI), it was necessary to devise a means of dissolving the sample so as to prevent any air oxidation of the uranium(IV) to uranium(VI). For this determination, the conventional potassium dichromate volumetric method was used except that the sample was dissolved under reflux in 7 M H/sub 3/PO/sub 4/ which contained an excess of standard dichromate solution. Following the dissolution of the sample, this excess was determined by back titration with a standard solution of iron(II). Barium diphenylaminesulfonate was used as the indicator. Initial tests on the dissolution of samples of thorium oxide-uranium oxide in hot HC1O/sub 4/ and hot HCI are described. (auth)

Research Organization:
Oak Ridge National Lab., Tenn.
NSA Number:
NSA-15-002584
OSTI ID:
4117883
Report Number(s):
CF-59-4-40
Country of Publication:
United States
Language:
English

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