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RECOIL STUDIES OF NUCLEAR REACTIONS INDUCED BY HEAVY IONS

Journal Article · · Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D
The mechanism of nuclear reactions induced by heavy ions was investigated by measuring the recoil ranges of Tb/sup 149/, At/sup 211/, and other alpha emitting isotopes of At and neighboring elements and by determining the cross sections for the formation of Tb/sup 149/ and At/sup 211/. Recoil ranges wer e consistent with compound-nucleus formation at all energies studied for the following reactions: Pr/sup 141/(C/sup 12/,4n)Tb/sup 1/ >s/sup 49/, Ce(N/ sup 14/.xn)Tb/sup 149/, La/sup 139/(O/sup 18/,bn)Tb/sup 1/ >s/sup 49/, La/sup 139/ (8/sup >/8n)Tbitl. and Ba(Ne/sup 22/.pxn)Tb/sup 149/. A similar result was obtained for th e reaction Pr/sup 141/(O/sup 16/,2p6n)Tb/sup 149/ at 138 and 14 6 Mev and for the reactions Au/sup 197/(O/sup 16/,2pxn, and 3pxn)At, Po at energies b elow 100 Mev. The excitation functions of the (HI.xn)Tb/sup 149/ reactions seemed to be characteristic of an evaporation process but had smaller peak cross sections than did the excitation functions of the reactions Ba(Ne/sup 22/,pxn)Tb/ sup 149/ or Pr/sup 1/ /sup 41/(O/sup 16/. 2p6n)Tb/sup 149/. It was concluded that most reactions probably involve charged-particle emission. The reaction Ba(Ne/sup 22/ pxn)Tb/sup 149/ seemed to occur with much greater probability than the reaction Ba(Ne/sup 20/,pxn)Tb/sup 149/. In many cases the compound-nucleus mechanism could not account for the results. Partial momentum transfer was observed in the reactions Au/sup 197/(O/sup 16/,2pxn, and 3pxn)At, Po at enengies above 100 Mev. Partial momentum transfer also occurred when Bi was bombarded at energies 1.3 times the barrier energy or greater. Reactions ot Bi with heavy ions (Ne/sup 20/ is a possible exception) at energies near the Coulomb barrier produced At/sup 211/ with greater recoil energy than expected from a compound- nucleus mechanism. Apparently particles were emitted in the backward direction. Near the barrier the cross section for the production of At/sup 211/ by C/sup 12/ , O/sup 1/ s/sup 6/, and Ne/sup 20/ bombardment comprised about one-fourth the value calculated for compound-nucleus formation. Therefore. the cross section for all noncompound-nucleus reactions must comprise a large fraction of the total interaction cross section. The experiments with Pb as a target were also consistent with this conclusion. (auth)
Research Organization:
Univ. of California, Berkeley
NSA Number:
NSA-15-010063
OSTI ID:
4086892
Report Number(s):
UCRL-9118; 0031-899X
Journal Information:
Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D, Journal Name: Physical Review (U.S.) Superseded in part by Phys. Rev. A, Phys. Rev. B: Solid State, Phys. Rev. C, and Phys. Rev. D Vol. Vol: 121; ISSN PHRVA
Country of Publication:
United States
Language:
English

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