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PREPARATION OF LONG-LIVED TERBIUM-157 AND TERBIUM-158

Journal Article · · J. Inorg. & Nuclear Chem.

A 5-mg sample of dysprosium oxide enriched to 13.8% in Dy/sup 156/ was irradiated with neutrons in the Materials Testing Reactor. The sample received an exposure of 2 x 10/sup 21/ neutrons/cm/sup 2/ over a three-month interval. Four months after irradiation, mass analysis was made of the unseparated sample. The presence of mass peaks at 157, 159, 165, and 166, unobservable in the sample before irradiation, indicated neutron capture in Dy/sup 156/, Dy/sup 158/, and Dy/ sup 16/< s4>s. The samples were chemically fractionated, and scintillation spectroscopy were chemically fractionated, and scintillation spectroscopy revealed the presence of Ho/sup 166/, Dy/sup 159/, and Tb/sup 16/< s0>s. Mass- spectrometric investigation of the terbium fraction revealed the existence of mass peaks at 157, 158, 159, and 160, indicating the preparation of new long- lived isotopes Tb/sup 157/and Tb/sup 158/ s. Calculations indicated that the K- capture half lives of these isotopes are greater than 30 and 15 years, respectively. (M.C.G.)

Research Organization:
Univ. of California, Berkeley
NSA Number:
NSA-15-010995
OSTI ID:
4086560
Report Number(s):
UCRL-9287
Journal Information:
J. Inorg. & Nuclear Chem., Journal Name: J. Inorg. & Nuclear Chem. Vol. Vol: 16
Country of Publication:
United States
Language:
English

References (5)

Hyperfine Structure and Nuclear Moments of Gadolinium journal March 1956
Neutron-Deficient Activities of Terbium journal September 1955
Hyperfine Structure and Nuclear Moments of Gadolinium from Paramagnetic Resonance Spectrum journal September 1956
Nuclear Spectroscopy of Neutron-Deficient Rare Earths (Tb through Hf) journal November 1957
Isomeric Transitions in the Rare-Earth Elements journal June 1957

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