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Interface degradation in CAS/Nicalon during elevated temperature aging

Conference ·
OSTI ID:39120
 [1]; ;  [2]
  1. Oak Ridge National Lab., TN (United States)
  2. Univ. of Warwick, Coventry (United Kingdom). Centre for Advanced Materials Technology

A CaO-Al{sub 2}O{sub 3}-SiO{sub 2} (CAS)/Nicalon glass-ceramic matrix composite has been subjected to elevated temperature oxidation heat-treatments between 375 and 1200{degrees}C, for up to 100 hours. Micro- and macro-mechanical properties have been determined by fiber push-down, using a mechanical properties microprobe, and flexure testing, respectively. Aging between 450 and 800{degrees}C results in significant property degradation, with reduced bending modulus and flexure strength, increased fiber sliding stress, and a transition to a purely brittle failure mode. Aging degradation is due to oxidative removal of the carbon interlayer, with the subsequent formation of a silica bond between fiber and matrix. At higher temperatures, carbon is retained due to the formation of a protective silica plug at exposed fiber ends, with the subsequent retention of composite properties. Short duration pre-treatment schedules, at 1000 or 1100{degrees}C, were developed to prevent intermediate temperature property degradation.

Research Organization:
Oak Ridge National Lab., TN (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States); European Economic Community, Brussels (Belgium)
DOE Contract Number:
AC05-84OR21400
OSTI ID:
39120
Report Number(s):
CONF-941144--115; ON: DE95008843
Country of Publication:
United States
Language:
English