Magnetocaloric effect observations near room temperature in few-layered chromium telluride (Cr2Te3)

Tiwari, Nishant; Gowda, Chinmayee Chowde; Mishra, Subhendu; Pandey, Prafull; Talapatra, Saikat; Chaudhary, Varun; Singh, Abhishek K.; Tiwary, Chandra Sekhar

doi:10.1039/D5NR04469C

Magnetocaloric effect observations near room temperature in few-layered chromium telluride (Cr₂Te₃)

Journal Article · Fri Dec 05 00:00:00 EST 2025 · Nanoscale

DOI:https://doi.org/10.1039/D5NR04469C· OSTI ID:3021128

Tiwari, Nishant ^[1]; ^[1]; Mishra, Subhendu ^[2]; Pandey, Prafull ^[3]; Talapatra, Saikat ^[4]; ^[5]; ^[2]; ^[1]

Indian Institute of Technology Kharagpur, West Bengal (India)
Indian Institute of Science, Karnataka (India)
Indian Institute of Technology Gandhinagar, Gujarat (India)
Southern Illinois University, Carbondale, IL (United States)
Chalmers University of Technology, Gothenburg (Sweden)

Transition metal telluride compositions are explored extensively for their unique magnetic behavior. Few-layered chromium telluride (Cr₂T_e3) exhibits a near-room-temperature phase transition, where the material can be effectively used in applications such as magnetic refrigeration. Compared to existing magnetocaloric materials, Heusler alloys, and rare-earth-based alloys, the large-scale synthesis of mechanically exfoliated Cr₂Te₃ involves less complexity, resulting in a stable composition. Compared to existing tellurides, Cr₂Te₃ exhibited a large change in magnetic entropy (|ΔS_M|) of 1.88 J k^g−1 K⁻¹ at a magnetic field of 4 T. A refrigeration capacity (RC) of ∼82 J kg⁻¹ was determined from the change in magnetic entropy versus temperature curve. The results were comparable with those for existing Cr-based compounds. First-principles density functional theory (DFT) confirmed the magnetic properties of Cr₂Te₃, including a near-room-temperature Curie temperature, T_C, consistent with experimental results. Here, structural transition was also observed using first-principles DFT, which is responsible for the magnetic behavior.

View Accepted Manuscript (DOE)

Research Organization:: Southern Illinois University, Carbondale, IL (United States)

Sponsoring Organization:: Asian Office of Aerospace Research and Development (AOARD); USDOE

Grant/Contract Number:: FG02-06ER46291

Other Award/Contract Number:: FA2386-21-1-4014

OSTI ID:: 3021128

Journal Information:: Nanoscale, Journal Name: Nanoscale Journal Issue: 4 Vol. 18; ISSN 2040-3364; ISSN 2040-3372

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United States

Language:: English

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