Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Mass of 101Sn and Bayesian extrapolations to the proton drip line

Journal Article · · Physical Review. C
DOI:https://doi.org/10.1103/vck7-1c4t· OSTI ID:3018617
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [1];  [1];  [1];  [3];  [3];  [1];  [1];  [3];  [2];  [2];  [4];  [5] more »;  [6];  [1];  [1];  [1];  [7];  [1] « less
  1. Michigan State University, East Lansing, MI (United States)
  2. University of Notre Dame, IN (United States)
  3. Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
  4. Michigan State University, East Lansing, MI (United States); University of Zagreb (Croatia)
  5. Michigan State University, East Lansing, MI (United States); Central Michigan University, Mount Pleasant, MI (United States)
  6. Universität Erlangen (Germany)
  7. Argonne National Laboratory (ANL), Argonne, IL (United States)
The favorable energy configurations of nuclei at magic numbers of 𝑁 neutrons and 𝑍 protons are fundamental for understanding the evolution of nuclear structure. The 𝑍 = 50 (tin) isotopic chain is a frontier for such studies, with particular interest at and around the doubly magic 100Sn isotope, for which the mass is a topic of debate. Precise mass values for neutron-deficient isotopes provide necessary anchor points for mass models to test extrapolations near the proton drip line, where experimental studies remain out of reach. In this work, we report a Penning trap mass measurement of 101Sn . The determined mass excess of −59889.89⁢(96) keV for 101Sn represents a factor-of-300 improvement over the current precision and indicates that 101Sn is less bound than previously thought. Mass predictions from a recently developed Bayesian model combination framework employing statistical machine learning and nuclear masses computed within seven global models based on nuclear density functional theory agree within 1⁢𝜎 with experimental masses from the 48 ≤ 𝑍 ≤ 52 isotopic chains. The framework's resilience to new mass data gave confidence in the extrapolation of tin masses down to 𝑁 = 46. Our calculations suggest that 96Sn is a two-proton drip line nucleus and predict a mass excess of −58090⁢(800) keV for 100Sn , showing a preference within 1⁢𝜎 for the mass of 100Sn derived from the 𝛽-delayed 𝑄 value measured at GSI.
Research Organization:
Michigan State University; Michigan State University, East Lansing, MI (United States)
Sponsoring Organization:
U.S. National Science Foundation; USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF); USDOE Office of Science (SC), High Energy Physics (HEP); USDOE Office of Science (SC), Nuclear Physics (NP)
Grant/Contract Number:
AC02-05CH11231; AC02-06CH11357; NA0003960; NA0004074; SC0013365; SC0018362; SC0022538; SC0023175; SC0023633; SC0023688
Other Award/Contract Number:
PHY-2111185
PHY-2310059
OSTI ID:
3018617
Alternate ID(s):
OSTI ID: 3015603
OSTI ID: 3029799
Journal Information:
Physical Review. C, Journal Name: Physical Review. C Journal Issue: 2 Vol. 113; ISSN 2469-9985; ISSN 2469-9993
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (71)

A phase-imaging technique for cyclotron-frequency measurements journal September 2013
Principal components of nuclear mass models journal May 2024
Neutron Single-Particle States in 101Sn by Polynomial Fits and Shell Model Calculations for Light Sn Isotopes journal November 2023
Experimental approach towards shell structure at 100Sn and 78Ni journal June 2002
Analysis methods and code for very high-precision mass measurements of unstable isotopes journal October 2021
A “Lorentz” steerer for ion injection into a Penning trap journal May 2007
The LEBIT 9.4T Penning trap mass spectrometer
  • Ringle, R.; Bollen, G.; Prinke, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 604, Issue 3 https://doi.org/10.1016/j.nima.2009.03.207
journal June 2009
The LEBIT ion cooler and buncher
  • Schwarz, S.; Bollen, G.; Ringle, R.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 816 https://doi.org/10.1016/j.nima.2016.01.078
journal April 2016
A laser ablation source for offline ion production at LEBIT journal June 2016
Improving the measurement sensitivity of the Canadian Penning Trap mass spectrometer through PI-ICR journal January 2020
Online tests of the Advanced Cryogenic Gas Stopper at NSCL journal January 2020
Commissioning of the Advanced Rare Isotope Separator ARIS at FRIB journal July 2023
Proton decay of 108I and its significance for the termination of the astrophysical rp-process journal May 2019
Isomer studies in the vicinity of the doubly-magic nucleus 100Sn: Observation of a new low-lying isomeric state in 97Ag journal March 2020
An alternative viewpoint on the nuclear structure towards 100Sn: Lifetime measurements in 105Sn journal October 2023
Shell structure of exotic nuclei journal July 2007
The structure of 100Sn and neighbouring nuclei journal March 2013
Superallowed Gamow–Teller decay of the doubly magic nucleus 100Sn journal June 2012
Evidence of a sudden increase in the nuclear size of proton-rich silver-96 journal July 2021
Mass measurements of 99–101In challenge ab initio nuclear theory of the nuclide 100Sn journal September 2021
Precision mass measurement of lightweight self-conjugate nucleus 80Zr journal November 2021
Electromagnetic properties of indium isotopes illuminate the doubly magic character of 100Sn journal September 2024
Local Bayesian Dirichlet mixing of imperfect models journal November 2023
The accuracy of heavy‐ion mass measurements using time of flight‐ion cyclotron resonance in a Penning trap journal November 1990
Bayes Factors journal June 1995
The shell model at 100 Sn—An experimental status report journal January 1995
The generator coordinate method and quantised collective motion in nuclear systems journal January 1987
The AME 2020 atomic mass evaluation (II). Tables, graphs and references* journal March 2021
Beyond the proton drip line: Bayesian analysis of proton-emitting nuclei journal January 2020
Quantified limits of the nuclear landscape journal April 2020
Spectroscopy of Cd 99 and In 101 from β decays of In 99 and Sn 101 journal July 2020
Effective shell-model interaction for nuclei “southeast” of Sn100 journal December 2021
Isochronous mass measurements of neutron-deficient nuclei from Sn112 projectile fragmentation journal January 2023
Nucleonic shells and nuclear masses journal April 2024
Uncertainty quantification of mass models using ensemble Bayesian model averaging journal May 2024
High-precision mass measurement of Sn103 restores smoothness of the mass surface journal January 2025
Refining the nuclear mass surface with the mass of Sn 103 journal January 2025
Variations in the charge radii of indium isotopes between N=52 and 82 journal June 2025
Proton-rich exotic heavy nuclei: Self-consistent calculations journal July 1988
Resolution of nuclear ground and isomeric states by a Penning trap mass spectrometer journal December 1992
Limits of proton stability nearSn100 journal March 1995
Shape coexistence and the effective nucleon-nucleon interaction journal June 1999
New relativistic mean-field interaction with density-dependent meson-nucleon couplings journal February 2005
High-precision Penning trap mass measurements of Ca 37 , 38 and their contributions to conserved vector current and isobaric mass multiplet equation journal May 2007
Microscopic justification of the equal filling approximation journal July 2008
Relativistic nuclear energy density functionals: Adjusting parameters to binding energies journal September 2008
Nuclear energy density optimization: Large deformations journal February 2012
Nuclear energy density optimization: Shell structure journal May 2014
Toward a global description of nuclear charge radii: Exploring the Fayans energy density functional journal June 2017
Bayesian approach to model-based extrapolation of nuclear observables journal September 2018
Optimizing the relativistic energy density functional with nuclear ground state and collective excitation properties journal March 2019
Why Is Sideband Mass Spectrometry Possible with Ions in a Penning Trap? journal April 2009
Quenching of the SnSbTe Cycle in the r p Process journal June 2009
Orbital Dependent Nucleonic Pairing in the Lightest Known Isotopes of Tin journal October 2010
Phase-Imaging Ion-Cyclotron-Resonance Measurements for Short-Lived Nuclides journal February 2013
Structure of the Lightest Tin Isotopes journal April 2018
Novel Shape Evolution in Sn Isotopes from Magic Numbers 50 to 82 journal August 2018
Neutron Drip Line in the Ca Region from Bayesian Model Averaging journal February 2019
Improved Value for the Gamow-Teller Strength of the Sn 100 Beta Decay journal June 2019
Mass Measurement of 100 Sn journal September 1996
Single-Neutron States in Sn 101 journal July 2007
Model orthogonalization and Bayesian forecast mixing via principal component analysis journal September 2024
Reevaluation of X-Ray Atomic Energy Levels journal January 1967
Evolution of shell structure in exotic nuclei journal March 2020
Measurements of β -delayed proton emitters in the region of Sn100 journal September 2025
Lattice Calculation of the Sn Isotopes near the Proton Dripline journal February 2026
Charge Radii Measurements of Exotic Tin Isotopes in the Proximity of N = 50 and N = 82 journal November 2025
Study of radial motion phase advance during motion excitations in a Penning trap and accuracy of JYFLTRAP mass spectrometer journal November 2021
First application of the phase-imaging ion-cyclotron resonance technique at TRIGA-Trap journal February 2023
Accelerator commissioning and rare isotope identification at the Facility for Rare Isotope Beams journal March 2022
Trends in the Structure of Nuclei near 100Sn journal March 2022