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Nuclear forensic analysis on uranium ore concentrates: A multi-laboratory intercomparison study

Journal Article · · Journal of Radioanalytical and Nuclear Chemistry
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  1. Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
  2. Japan Atomic Energy Agency (JAEA), Tokai (Japan)
  3. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
  4. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
A collaboration between the United States and Japan performed nuclear forensic analyses on a set of 7 uranium ore concentrate (UOC) samples with known origins to improve methodologies and best practices in the field. Overall, good agreement between the 4 participating laboratories was achieved for uranium assay, uranium isotope composition, strontium isotope composition, and trace element analysis. In conclusion, the combination of these four signatures is sufficient to distinguish the different origins among these studied UOCs.
Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC52-07NA27344
OSTI ID:
3012086
Report Number(s):
LLNL--JRNL-2007303
Journal Information:
Journal of Radioanalytical and Nuclear Chemistry, Journal Name: Journal of Radioanalytical and Nuclear Chemistry Journal Issue: 12 Vol. 334; ISSN 1588-2780; ISSN 0236-5731
Publisher:
SpringerCopyright Statement
Country of Publication:
United States
Language:
English

References (25)

Anion analysis in uranium ore concentrates by ion chromatography journal March 2009
Identification of uranium signatures relevant for nuclear safeguards and forensics journal April 2017
Application of the 226Ra–230Th–234U and 227Ac–231Pa–235U radiochronometers to uranium certified reference materials journal November 2017
Collaborative Study for Certification of Trace Elements in Uranium Ore Concentrate CRMs UCLO-1, UCHI-1, and UPER-1 journal September 2022
Separation and preconcentration of uranium from acidic media by extraction chromatography journal August 1992
Radiogenic isotopes: systematics and applications to earth surface processes and chemical stratigraphy journal May 2004
The provenance of Australian uranium ore concentrates by elemental and isotopic analysis journal April 2008
Trace element and U isotope analysis of uraninite and ore concentrate: Applications for nuclear forensic investigations journal September 2017
Molybdenum isotope compositions of uranium ore concentrates by double spike MC-ICP-MS journal April 2019
In-situ production of natural 236U in groundwaters and ores in high-grade uranium deposits journal September 2015
Natural variations in uranium isotope ratios of uranium ore concentrates: Understanding the 238U/235U fractionation mechanism journal March 2010
Rhenium Isotope Reconnaissance of Uranium Ore Concentrates journal October 2024
Nuclear forensic analysis of an unknown uranium ore concentrate sample seized in a criminal investigation in Australia journal July 2014
Uranium isotopic compositions of the crust and ocean: Age corrections, U budget and global extent of modern anoxia journal October 2015
The state of nuclear forensics journal January 2013
Application of neodymium isotope ratio measurements for the origin assessment of uranium ore concentrates journal November 2014
Samarium isotope compositions of uranium ore concentrates: A novel nuclear forensic signature journal January 2021
Determining provenance of uranium ore concentrates using 143Nd/144Nd journal November 2022
Trends and perspectives in Nuclear Forensic Science journal January 2022
Application of Lead and Strontium Isotope Ratio Measurements for the Origin Assessment of Uranium Ore Concentrates journal October 2009
Alpha-Recoil Thorium-234: Dissolution into Water and the Uranium-234/Uranium-238 Disequilibrium in Nature journal July 1971
A 35-million-year record of seawater stable Sr isotopes reveals a fluctuating global carbon cycle journal March 2021
Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control journal June 2016
Investigation of the 236 U/ 238 U isotope abundance ratio in uranium ores and yellow cake samples journal March 2011
Analysis of uranium ore concentrates for origin assessment journal September 2011

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