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First 𝛽-Delayed Two-Neutron Spectroscopy of the 𝑟-Process Nucleus 134In and Observation of the 𝑖13/2 Single-Particle Neutron State in 133Sn

Journal Article · · Physical Review Letters
DOI:https://doi.org/10.1103/l24v-5m31· OSTI ID:3003798
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  1. University of Tennessee
  2. University of Tokyo
  3. University of Warsaw
  4. Lawrence Livermore National Laboratory
  5. CSIC-Universidad de Valencia
  6. University of York
  7. University of Warsaw; National Centre for Nuclear Research
  8. iThemba LABS
  9. Universidad Complutense de Madrid
  10. CSIC
  11. KU Leuven
  12. Horia Hulubei National Institute for Physics and Nuclear Engineering
  13. University of York; University of Edinburgh
  14. Aarhus University
  15. University of Liverpool
  16. Los Alamos National Lab
  17. STFC Daresbury Laboratory
  18. Horia Hulubei National Institute of Physics and Nuclear Engineering (IFIN-HH)
  19. CERN
  20. University of the Western Cape
  21. University of Jyväskylä; University of Helsinki
  22. University of Tennessee; Universidad Complutense de Madrid; Warsaw University
  23. University of Surrey
  24. Tennessee Technological University
  25. Institut Laue-Langevin; University of Jyväskylä
  26. Universität zu Köln
This manuscript reports on the direct observation of a 𝛽-delayed two-neutron emission in a study of 134In at the ISOLDE Decay Station using neutron spectroscopy. We also report on the first measurement in 𝛽 decay of the long-sought 13/2+ excited state in 133Sn, attributed to be the neutron single-particle 𝑖13/2 orbital. The observation of sequential neutron emission is used to extract the relative population of the 𝑖13/2 state, which was found to be much smaller than the predictions of the statistical model. The experiment was possible because of the innovative use of a neutron array with neutron discrimination and interaction tracking capabilities. This is the first study of the details of the two-neutron emission for a nucleus, which belongs to the 𝑟-process path. Understanding 𝛽-delayed two-neutron emission probabilities is essential to validate models used in astrophysical 𝑟-process nucleosynthesis calculations. Observing two-neutron emissions in 𝛽 decay paves the way for new experiments to study energy and angular correlations for 𝛽-delayed multineutron emitters.
Research Organization:
The University of Tennessee, Knoxville, TN (United States)
Sponsoring Organization:
USDOE
Contributing Organization:
IDS Collaboration
Grant/Contract Number:
89233218CNA000001; AC05-00OR22725; AC52-07NA27344; FG02-96ER40983; NA0002132; NA0004068
OSTI ID:
3003798
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 15 Vol. 135; ISSN 0031-9007; ISSN 1079-7114
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (35)

Properties of N=84, even-even nuclei populated in the spontaneous fission of 248Cm journal February 2000
Neutron single-particle energies in the 132Sn region journal July 1999
Local and global nucleon optical models from 1 keV to 200 MeV journal January 2003
Nuclear properties for astrophysical and radioactive-ion-beam applications (II) journal January 2019
A digital data acquisition framework for the Versatile Array of Neutron Detectors at Low Energy (VANDLE)
  • Paulauskas, S. V.; Madurga, M.; Grzywacz, R.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 737 https://doi.org/10.1016/j.nima.2013.11.028
journal February 2014
Performance of the Versatile Array of Neutron Detectors at Low Energy (VANDLE)
  • Peters, W. A.; Ilyushkin, S.; Madurga, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 836 https://doi.org/10.1016/j.nima.2016.08.054
journal November 2016
Conceptual design and first results for a neutron detector with interaction localization capabilities
  • Heideman, J.; Pérez-Loureiro, D.; Grzywacz, R.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 946 https://doi.org/10.1016/j.nima.2019.162528
journal December 2019
Neutron detection efficiency of the Neutron dEtector with Xn Tracking (NEXT)
  • Neupane, S.; Heideman, J.; Grzywacz, R.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 1020 https://doi.org/10.1016/j.nima.2021.165881
journal December 2021
Experimental tests of an advanced proton-to-neutron converter at ISOLDE-CERN journal October 2014
The impact of individual nuclear properties on r -process nucleosynthesis journal January 2016
The magic nature of 132Sn explored through the single-particle states of 133Sn journal May 2010
235 U(n, f) Independent fission product yield and isomeric ratio calculated with the statistical Hauser–Feshbach theory journal April 2018
Ion beam production and study of radioactive isotopes with the laser ion source at ISOLDE journal July 2017
The ISOLDE facility journal August 2017
The AME 2020 atomic mass evaluation (II). Tables, graphs and references* journal March 2021
The Mechanism of Nuclear Fission journal September 1939
The Inelastic Scattering of Neutrons journal July 1952
Strong one-neutron emission from two-neutron unbound states in β decays of the r -process nuclei Ga 86 , 87 journal September 2019
Extension of the Hauser-Feshbach fission fragment decay model to multichance fission journal January 2021
First β -decay spectroscopy of In135 and new β -decay branches of In134 journal October 2021
Uncertainty-quantified phenomenological optical potentials for single-nucleon scattering journal January 2023
β -delayed neutron spectroscopy of In133 journal July 2023
Evidence of nonstatistical neutron emission following β decay near doubly magic Sn132 journal August 2023
Gamow-Teller and first-forbidden decays near the r -process paths at N = 50 , 8 2 , and 126 journal February 2003
Calculation of delayed-neutron energy spectra in a quasiparticle random-phase approximation–Hauser-Feshbach model journal November 2008
Nuclear halo structure and pseudospin symmetry journal March 2010
Robust upper limit of the neutroni13/2single-particle energy journal October 2014
Large β -Delayed One and Two Neutron Emission Rates in the Decay of Ga 86 journal September 2013
Double-Magic Nature of Sn 132 and Pb 208 through Lifetime and Cross-Section Measurements journal April 2014
β -Delayed One and Two Neutron Emission Probabilities Southeast of Sn132 and the Odd-Even Systematics in r -Process Nuclide Abundances journal October 2022
In133 : A Rosetta Stone for Decays of r -Process Nuclei journal July 2023
Compound-Nucleus and Doorway-State Decays of β -Delayed Neutron Emitters K51,52,53 journal July 2024
First Observation of Beta-Delayed Two-Neutron Radioactivity: Li 11 journal November 1979
Detailed Spectroscopy of the Doubly Closed Shell Nucleus S n : 132 First Observation of Octupole Collectivity journal October 1994
Single-Neutron States in S 133 n journal August 1996