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High-power broadly tunable picosecond IR laser system for use in nonlinear spectroscopic applications

Journal Article · · Journal of the Optical Society of America, Part B: Optical Physics
; ;  [1];  [2]
  1. Department of Chemistry, University of Oregon, Eugene, Oregon 97403 (United States)
  2. Shared Laser Facility, University of Oregon, Eugene, Oregon 97403 (United States)

We developed a high-power tunable picosecond IR laser system suitable for nonlinear spectroscopic investigations. We employ a Ti:sapphire regenerative amplifier that produces 1.9-ps, 17-cm{sup {minus}1}, 800-nm pulses at 1 kHz as a pump source. White-light generation in ethylene glycol and optical parametric amplification in potassium titanyl phosphate are used to produce the IR pulses. The tuning range extends from 2.4 to 3.8 {mu}m in the idler and 1.0 to 1.2 {mu}m in the signal. A total efficiency (signal plus idler) as high as 20{percent} was achieved. The spatial, spectral, and temporal characteristics of the IR beam are presented along with vibrational sum-frequency spectra from a glass/octadecyltrichlorosilane/air interface. {copyright} {ital 1996 Optical Society of America.}

OSTI ID:
286941
Journal Information:
Journal of the Optical Society of America, Part B: Optical Physics, Journal Name: Journal of the Optical Society of America, Part B: Optical Physics Journal Issue: 9 Vol. 13; ISSN JOBPDE; ISSN 0740-3224
Country of Publication:
United States
Language:
English

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