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Photoelectron spectroscopy of laser-excited surfaces by synchrotron radiation

Journal Article · · Journal of the Optical Society of America, Part B: Optical Physics
 [1];  [2];  [1]
  1. Naval Research Laboratory, Washington, D.C. 20375 (United States)
  2. Fritz-Haber Institute, Faradayweg 4-6, D-14195 Berlin (Germany)

Nanosecond pump{endash}probe photoelectron spectroscopy by means of synchrotron radiation from 6 to 130 eV anticipates the application of new short-wavelength sources with comparable photon energies but shorter pulse durations. The influence of pulsed-UV source characteristics on photoelectron spectrosocpy experiments on solid surfaces, including space-charge effects, is examined. A resonant photoemission experiment is presented to illustrate the use of tunable photon energies in pump{endash}probe photoelectron spectroscopy involving core levels, and a new autoionizing resonance is reported in which electrons laser excited into a GaAs(110) surface state are emitted when a Ga 3{ital d} surface core exciton decays. {copyright} {ital 1996 Optical Society of America.}

DOE Contract Number:
AC02-76CH00016
OSTI ID:
278672
Journal Information:
Journal of the Optical Society of America, Part B: Optical Physics, Journal Name: Journal of the Optical Society of America, Part B: Optical Physics Journal Issue: 1 Vol. 13; ISSN JOBPDE; ISSN 0740-3224
Country of Publication:
United States
Language:
English

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