Ultrafast high-harmonic spectroscopy of solids

Heide, Christian; Kobayashi, Yuki; Haque, Sheikh Rubaiat Ul; Ghimire, Shambhu

doi:10.1038/s41567-024-02640-8

Ultrafast high-harmonic spectroscopy of solids

Journal Article · Thu Oct 10 00:00:00 EDT 2024 · Nature Physics

DOI:https://doi.org/10.1038/s41567-024-02640-8· OSTI ID:2587681

^[1]; ^[2]; ^[3]; ^[4]

SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Photon Ultrafast Laser Science and Engineering Institute (PULSE); Stanford Univ., CA (United States)
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Photon Ultrafast Laser Science and Engineering Institute (PULSE); Univ. of Michigan, Ann Arbor, MI (United States)
Stanford Univ., CA (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Photon Ultrafast Laser Science and Engineering Institute (PULSE)

High-harmonic spectroscopy, an ultrafast all-optical technique initially conceptualized in atomic and molecular systems, has now emerged as a powerful platform for studying the structure and dynamics of condensed matter. Unlike that in the gas phase, solid-state high-harmonic generation relies on the fundamental response from high atomic density and periodicity, leading to interband transitions and coherent driving of electrons and holes in their respective bands. These mechanisms make high-harmonic spectroscopy particularly sensitive to the electronic band structure, topological properties and many-body correlations in condensed media. An advantage of high-harmonic spectroscopy over other spectroscopic methods is its ability to probe ultrafast phenomena, capturing femto- to attosecond dynamics of multi-band and strongly correlated electron interactions in solids. Furthermore, in this Review, we discuss the latest experimental and theoretical advances in ultrafast high-harmonic spectroscopy of solids and provide perspectives for future research in this field.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 2587681

Journal Information:: Nature Physics, Journal Name: Nature Physics Journal Issue: 10 Vol. 20; ISSN 1745-2473; ISSN 1745-2481

Publisher:: Springer Science and Business Media LLCCopyright Statement

Country of Publication:: United States

Language:: English

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Ultrafast dephasing in solid-state high harmonic generation: macroscopic origin revealed by real-space dynamics [Invited] Brown, Graham G.; Jiménez-Galán, Álvaro; Silva, Rui E. F. Journal of the Optical Society of America B, Vol. 41, Issue 6 https://doi.org/10.1364/JOSAB.513543	journal	May 2024
Time-resolved high harmonic spectroscopy of dynamical symmetry breaking in bi-circular laser fields: the role of Rydberg states Jiménez-Galán, Álvaro; Zhavoronkov, Nickolai; Schloz, Marcel Optics Express, Vol. 25, Issue 19 https://doi.org/10.1364/OE.25.022880	journal	January 2017
Nonlinear propagation effects in high harmonic generation in reflection and transmission from gallium arsenide Xia, Peiyu; Kim, Changsu; Lu, Faming Optics Express, Vol. 26, Issue 22 https://doi.org/10.1364/OE.26.029393	journal	January 2018
Laser waveform control of extreme ultraviolet high harmonics from solids You, Yong Sing; Wu, Mengxi; Yin, Yanchun Optics Letters, Vol. 42, Issue 9 https://doi.org/10.1364/OL.42.001816	journal	January 2017
Characterization of high-harmonic emission from ZnO up to 11 eV pumped with a Cr:ZnS high-repetition-rate source Vampa, Giulio; Vasilyev, Sergey; Liu, Hanzhe Optics Letters, Vol. 44, Issue 2 https://doi.org/10.1364/OL.44.000259	journal	January 2019
Asymmetric single-cycle control of valence electron motion in polar chemical bonds Morimoto, Yuya; Shinohara, Yasushi; Tani, Mizuki Optica, Vol. 8, Issue 3 https://doi.org/10.1364/OPTICA.414213	journal	January 2021
Probing electron-hole coherence in strongly driven 2D materials using high-harmonic generation Heide, Christian; Kobayashi, Yuki; Johnson, Amalya C. Optica, Vol. 9, Issue 5 https://doi.org/10.1364/OPTICA.444105	journal	May 2022
High-harmonic generation with a twist: all-optical characterization of magic-angle twisted bilayer graphene Molinero, Eduardo B.; Datta, Anushree; Calderón, M. J. Optica, Vol. 11, Issue 2 https://doi.org/10.1364/OPTICA.510789	journal	January 2024
High-harmonic generation from artificially stacked 2D crystals Heide, Christian; Kobayashi, Yuki; Johnson, Amalya C. Nanophotonics, Vol. 12, Issue 2 https://doi.org/10.1515/nanoph-2022-0595	journal	January 2023
Polarization Flipping of Even-Order Harmonics in Monolayer Transition-Metal Dichalcogenides Kobayashi, Yuki; Heide, Christian; Kelardeh, Hamed Koochaki Ultrafast Science, Vol. 2021 https://doi.org/10.34133/2021/9820716	journal	August 2021

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