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Carbon nanotube nanofluidics

Journal Article · Thu Aug 07 00:00:00 EDT 2025 · Chemical Society Reviews

DOI:https://doi.org/10.1039/d5cs00233h· OSTI ID:2587410

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Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Univ. of California, Merced, CA (United States)

Fluid flow under extreme spatial confinement exhibits unusual physical behaviors. This nanofluidic transport regime is relevant to a variety of mass transport, separation, and energy production processes in biological and industrial systems. Carbon nanotubes (CNTs) offer a nearly ideal platform for exploring nanofluidic transport because of their extremely narrow, smooth, hydrophobic inner pores, which enable very fast molecular flow while providing strong selectivity. In this review, we aim to provide a comprehensive understanding of nanofluidics in CNTs, focusing on the basic physics of mass transport in CNTs, various experimental platforms developed to investigate these phenomena, and key results on the permeation of water, protons, and ions. We focus on the critical factors that influence transport efficiency and selectivity, such as slip flow and charge regulation in CNTs, and the roles of entrance effects, dehydration processes and ion–charge interactions at the CNT entrances. We also explore the confinement effects, highlighting how the unique one-dimensional structure of CNTs imposes distinct constraints on fluid behavior and leads to novel single-file transport phenomena. Finally, we address current challenges and future directions of CNT nanofluidics.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC52-07NA27344; SC0019112

OSTI ID:: 2587410

Report Number(s):: LLNL--JRNL-872513

Journal Information:: Chemical Society Reviews, Journal Name: Chemical Society Reviews Journal Issue: 19 Vol. 54; ISSN 1460-4744; ISSN 0306-0012

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United States

Language:: English

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