Review of honeycomb-based Kitaev materials with zigzag magnetic ordering

Garlea, Vasile Ovidiu; Sarkis, Colin L.

doi:10.1107/S2052520624009831

Review of honeycomb-based Kitaev materials with zigzag magnetic ordering

Journal Article · Sun Jan 19 23:00:00 EST 2025 · Acta Crystallographica. Section B, Structural Science, Crystal Engineering and Materials (Online)

DOI:https://doi.org/10.1107/S2052520624009831· OSTI ID:2573602

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Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

The search for a Kitaev quantum spin liquid in crystalline magnetic materials has fueled intense interest in the two-dimensional honeycomb systems. Many promising candidate Kitaev systems are characterized by a long-range-ordered magnetic structure with an antiferromagnetic zigzag-type order, where the static moments form alternating ferromagnetic chains. Recent experiments on high-quality single crystals uncovered the existence of intriguing multi-k magnetic structures, which evolved from zigzag structures. Those discoveries have sparked new theoretical developments and amplified interest in these materials. We present an overview of the honeycomb materials known to display this type of magnetic structure and provide detailed crystallographic information for the possible single- and multi-k variants.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2573602

Journal Information:: Acta Crystallographica. Section B, Structural Science, Crystal Engineering and Materials (Online), Journal Name: Acta Crystallographica. Section B, Structural Science, Crystal Engineering and Materials (Online) Journal Issue: 1 Vol. 81; ISSN 2052-5206

Publisher:: International Union of CrystallographyCopyright Statement

Country of Publication:: United States

Language:: English

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Neutron scattering in the proximate quantum spin liquid α-RuCl ₃ Banerjee, Arnab; Yan, Jiaqiang; Knolle, Johannes Science, Vol. 356, Issue 6342 https://doi.org/10.1126/science.aah6015	journal	June 2017
Quantum spin liquids Broholm, C.; Cava, R. J.; Kivelson, S. A. Science, Vol. 367, Issue 6475 https://doi.org/10.1126/science.aay0668	journal	January 2020
Half-integer quantized anomalous thermal Hall effect in the Kitaev material candidate α-RuCl ₃ Yokoi, T.; Ma, S.; Kasahara, Y. Science, Vol. 373, Issue 6554 https://doi.org/10.1126/science.aay5551	journal	July 2021
Quantum Phases in Two-Dimensional Frustrated Spin-1/2 Antiferromagnets Sindzingre, P.; Lhuillier, C.; Fouet, J. -B. International Journal of Modern Physics B, Vol. 17, Issue 28 https://doi.org/10.1142/S0217979203020168	journal	November 2003
Physics of the Kitaev Model: Fractionalization, Dynamic Correlations, and Material Connections Hermanns, M.; Kimchi, I.; Knolle, J. Annual Review of Condensed Matter Physics, Vol. 9, Issue 1 https://doi.org/10.1146/annurev-conmatphys-033117-053934	journal	March 2018
Symmetry-Based Computational Tools for Magnetic Crystallography Perez-Mato, J. M.; Gallego, S. V.; Tasci, E. S. Annual Review of Materials Research, Vol. 45, Issue 1 https://doi.org/10.1146/annurev-matsci-070214-021008	journal	July 2015
Design of Multifunctional Honeycomb Materials Seepersad, Carolyn Conner; Dempsey, Benjamin M.; Allen, Janet K. AIAA Journal, Vol. 42, Issue 5 https://doi.org/10.2514/1.9594	journal	May 2004
Magnetic Properties of A2Ni2TeO6 (A = K, Li): Zigzag Order in the Honeycomb Layers of Ni2+ Ions Induced by First and Third Nearest-Neighbor Spin Exchanges Vasilchikova, Tatyana; Vasiliev, Alexander; Evstigneeva, Maria Materials, Vol. 15, Issue 7 https://doi.org/10.3390/ma15072563	journal	March 2022

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36 MATERIALS SCIENCE
Kitaev physics
QSLs
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magnetic structures
neutron diffraction
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Review of honeycomb-based Kitaev materials with zigzag magnetic ordering

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