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Material extrusion with integrated compression molding of NdFeB/SmFeN nylon bonded magnets using small- and large-scale pellet-based 3D-printers

Journal Article · · Additive Manufacturing Letters
 [1];  [2];  [2];  [2];  [3];  [3];  [2];  [1]
  1. Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Institute for Advanced Composites Manufacturing Innovation (IACMI), Knoxville, TN (United States)
  2. Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
  3. Ames Laboratory (AMES), Ames, IA (United States)
High-density bonded rare-earth magnets are manufactured using pellet-fed additive manufacturing (AM)/material extrusion and an integrated additive manufacturing-compression molding (AM-CM) process. Neodymium iron boron – samarium iron nitride in polyamide 12 (NdFeB-SmFeN/PA12) of 93 % weight fraction (65 % volume fraction) are used for the study. The mechanical properties (tensile strength and modulus), magnetic properties (maximum energy density, coercivity, remanence) are reported. Manufacturing parameters such as layer height, barrel temperatures, screw speed and gantry feed rate are optimized to obtain the highest possible density of the magnets using a small-scale desktop material extrusion printer. Large scale integrated additive manufacturing-compression molding (AM-CM) is then utilized to increase the density of the magnets by reducing porosity defects common in the material extrusion process. The density of as-printed magnets was 5.2 g/cm3 with a BHmax value of 124.14 kJ/m3, tensile strength of 20 MPa and a modulus of 2 GPa. AM-CM increased the density of the compound by 5.5 % (5.49 g/cm3). The reduction in porosity was confirmed using X-ray tomography (XCT). Improvement in mechanical strength of the material was also observed, with an increase in tensile strength of 25 % (25.09 MPa) and increase in tensile modulus of 275 % (5.49 GPa). Scanning electron microscopy showed increased particle-matrix adhesion with the integrated AM-CM process.
Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Advanced Materials & Manufacturing Technologies Office (AMMTO); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Vehicle Technologies Office (VTO); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Wind Energy Technologies Office
Grant/Contract Number:
AC02-07CH11358; AC05-00OR22725
OSTI ID:
2573173
Journal Information:
Additive Manufacturing Letters, Journal Name: Additive Manufacturing Letters Vol. 13; ISSN 2772-3690
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (14)

Binder Jetting: A Novel NdFeB Bonded Magnet Fabrication Process journal April 2016
Manufacturing Processes for Permanent Magnets: Part II—Bonding and Emerging Methods journal February 2022
REE Recovery from End-of-Life NdFeB Permanent Magnet Scrap: A Critical Review journal September 2016
A novel additive manufacturing compression overmolding process for hybrid metal polymer composite structures journal April 2023
High-performance molded composites using additively manufactured preforms with controlled fiber and pore morphology journal January 2021
Fused filament fabrication of Nd-Fe-B bonded magnets: Comparison of PA12 and TPU matrices journal February 2021
Effect of process on the magnetic properties of bonded NdFeB magnet journal April 2006
Studies on in situ magnetic alignment of bonded anisotropic Nd-Fe-B alloy powders journal January 2017
Mechanical properties of components fabricated with open-source 3-D printers under realistic environmental conditions journal June 2014
Compression molding of anisotropic NdFeB bonded magnets in a polycarbonate matrix journal September 2021
Additive manufacturing of highly dense anisotropic Nd–Fe–B bonded magnets journal July 2020
Packing bimodal magnetic particles to fabricate highly dense anisotropic rare earth bonded permanent magnets journal January 2023
A Threshold Selection Method from Gray-Level Histograms journal January 1979
Rare earth elements: Mendeleev’s bane, modern marvels journal January 2019

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