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Predicting Thermoset Resin Cure Kinetics for Composite Processing

Technical Report ·
DOI:https://doi.org/10.2172/2570004· OSTI ID:2570004
 [1];  [2]
  1. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Univ. of Oregon, Eugene, OR (United States)
  2. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Predicting a material’s thermal properties is not only useful for designing parts but also for defining processing parameters. This is especially applicable to wet-filament winding operations and the production of composite parts using thermoset res ins. For these, the formation of cross-linking bonds is affected by time and temperature, but the degree of cross-linking can be modeled using phenomenological methods. In the current study, the Kissinger and Flynn/Wall/Ozawa methods were both used to calculate kinetic parameters and produced values that were in agreement with each other. The kinetic parameters activation energy (Ea) and pre-exponential factor (𝐴) calculated from exothermic peak data increased between an epoxy and resole phenol resin system, with a cyanate ester having the highest. The successful application of both methods suggests applicability to future studies for developing cure recipes.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
DOE Contract Number:
89233218CNA000001
OSTI ID:
2570004
Report Number(s):
LA-UR--25-25454
Country of Publication:
United States
Language:
English

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