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Spin fluctuation driven magnetoresistance, domain Re-distribution and anomalous Hall effect in helical antiferromagnetic Eu metal thin films

Journal Article · · AIP Advances
DOI:https://doi.org/10.1063/9.0000861· OSTI ID:2528100
Europium (Eu) metal has a body centered cubic crystal structure which, upon a paramagnetic-to-helical magnetic phase transition, undergoes a body centered tetragonal distortion. The magnetic helix appears below a Néel temperature (TN) of ~90 K, and an applied magnetic field gives rise to conical magnet structure. We have prepared Eu metal thin films on Si (001) substrates using Eu metal as a target by pulsed laser deposition and studied the transport properties by a four-probe method. The resistance shows a sudden slope change at TN of 88 K. The magnetoresistance (MR) is positive at temperatures below 30 K and exhibits negative values above that. Our analyses show that the positive MR at low temperatures originates from magnetic field induced spin fluctuation, and the negative MR at higher temperature is a result of suppression of critical spin fluctuation of the Eu spins by the magnetic field. The Eu film also shows hysteretic MR behaviors in mid field range, which is a result of re-distribution of the helical antiferromagnetic domains by the magnetic fields. We have also studied the transverse magnetotransport in the Eu thin films. The observed anomalous Hall effect is believed to be associated with the magnetic moment induced by the field or due to the helical spin structure of Eu itself.
Research Organization:
University of Wyoming, Laramie, WY (United States)
Sponsoring Organization:
National Science Foundation (NSF); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
Grant/Contract Number:
SC0020074; SC0021281
OSTI ID:
2528100
Alternate ID(s):
OSTI ID: 2553075
Journal Information:
AIP Advances, Journal Name: AIP Advances Journal Issue: 3 Vol. 15; ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (42)

Neutron diffraction study of single crystal europium in an applied magnetic field journal August 1973
Magnetic and transport properties of non-equilibrium BCC EuFe alloys journal July 1997
Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature journal October 2015
Antiferromagnetic spintronics journal March 2016
Topological antiferromagnetic spintronics journal March 2018
Electrical switching of the topological anomalous Hall effect in a non-collinear antiferromagnet above room temperature journal March 2018
Anomalous Critical-Point Behavior in Europium Metal journal March 1969
Magnetic Properties of Rare‐Earth Metals and Alloys journal March 1965
Neutron Diffraction Studies on Europium Metal journal March 1962
Magnetostructural behavior in (110) europium films journal March 2008
Effect of the temperature history on the magnetism of (110) europium films journal March 2009
Anomalous magnetoresistance of nonequilibrium Eu-TM (Co, Mo) alloy thin films journal June 1998
Magnetic and transport properties of nonequilibrium Eu-Fe thin films journal June 1998
The theory of transport in helical spin-structure crystals journal November 2022
Anomalous Hall effect due to magnetic chirality in the pyrochlore lattice journal January 2009
Strong anisotropic anomalous Hall effect and spin Hall effect in the chiral antiferromagnetic compounds Mn 3 X ( X = Ge , Sn, Ga, Ir, Rh, and Pt) journal February 2017
Magnetic Susceptibility of Metallic Europium journal June 1960
Magnetic Structure of Europium journal July 1964
Hall Effect in Ferromagnetics journal September 1954
Anomalous and topological Hall effects in epitaxial thin films of the noncollinear antiferromagnet Mn 3 Sn journal March 2020
Transverse magnetoresistance in terbium and holmium single crystals journal May 1977
Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet journal September 2000
Rotation of magnetic propagation vectors induced by lattice clamping in (110)Eu films journal March 2005
Anomalous Hall effect due to spin chirality in the Kagomé lattice journal August 2006
Unconventional Anomalous Hall Effect in the Metallic Triangular-Lattice Magnet PdCrO 2 journal September 2010
Anomalous Hall Effect from Frustration-Tuned Scalar Chirality Distribution in Pr 2 Ir 2 O 7 journal July 2013
Anomalous Hall Effect Arising from Noncollinear Antiferromagnetism journal January 2014
Magnetic phase diagram of epitaxial dysprosium journal August 1993
Orbital Ferromagnetism and Anomalous Hall Effect in Antiferromagnets on the Distorted fcc Lattice journal August 2001
Topological Hall Effect and Berry Phase in Magnetic Nanostructures journal August 2004
Anomalous Hall effect in noncollinear antiferromagnetic Mn 3 NiN thin films journal September 2019
Hall Effect in Ferromagnetic Materials journal January 1953
Anomalous Hall effect journal May 2010
Antiferromagnetic spintronics journal February 2018
Magnetic configuration in [100] Eu films journal September 2003
Magnetoresistance of Antiferromagnetic Metals Due to s - d Interaction journal January 1973
Chirality-Driven Anomalous Hall Effect in Weak Coupling Regime journal November 2002
Magnetization Process of a Screw Spin System journal June 1962
Magnetization Process of a Screw Spin System. II journal January 1964
Magnetoresistance due to Electron-Spin Scattering in Antiferromagnetic Metals at Low Temperatures journal May 1973
Non-collinear antiferromagnets and the anomalous Hall effect journal December 2014
Magnetoelastic and Exchange Contributions to the Helical-Ferromagnetic Transition in Dysprosium Epitaxial Films journal July 1995

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