Autoionizing polaritons with the Jaynes-Cummings model

Cariker, Coleman; Yanez-Pagans, S.; Harkema, Nathan; Lindroth, Eva; Sandhu, Arvinder; Argenti, Luca

doi:10.1103/physreva.110.063119

Autoionizing polaritons with the Jaynes-Cummings model

Journal Article · Mon Dec 23 00:00:00 EST 2024 · Physical Review A

DOI:https://doi.org/10.1103/physreva.110.063119· OSTI ID:2500236

^[1]; ^[2]; Harkema, Nathan ^[2]; ^[3]; Sandhu, Arvinder ^[2]; ^[4]

University of Central Florida, Orlando, FL (United States); University of Arizona
University of Arizona, Tucson, AZ (United States)
Stockholm University (Sweden)
University of Central Florida, Orlando, FL (United States)

Intense laser pulses have the capability to couple resonances in the continuum, leading to the formation of a split pair of autoionizing polaritons. These polaritons can exhibit extended lifetimes due to interference between radiative and Auger decay channels. In this work we show how an extension of the Jaynes-Cummings model to autoionizing states quantitatively reproduces the observed phenomenology. Furthermore, this extended model allows us to study how the dressing laser parameters can be tuned to control the ionization rate of the polariton multiplet.

View Accepted Manuscript (DOE)

Research Organization:: University of Arizona, Tucson, AZ (United States)

Sponsoring Organization:: National Science Foundation's Theoretical AMO Physics; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0018251

OSTI ID:: 2500236

Alternate ID(s):: OSTI ID: 2506697

Journal Information:: Physical Review A, Journal Name: Physical Review A Journal Issue: 6 Vol. 110; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (57)

Atomic Resonance States and Their Role in Charge-Changing Processes Lindroth, Eva; Argenti, Luca Advances in Quantum Chemistry https://doi.org/10.1016/B978-0-12-397009-1.00005-9	book	January 2012
Tracing and controlling electronic dynamics in atoms and molecules by attosecond pulses Peng, Liang-You; Jiang, Wei-Chao; Geng, Ji-Wei Physics Reports, Vol. 575 https://doi.org/10.1016/j.physrep.2015.02.002	journal	April 2015
Optical fiber quantum biosensor based on surface plasmon polaritons for the label-free measurement of protein Peng, Yun; Zhao, Yong; Hu, Xu-guang Sensors and Actuators B: Chemical, Vol. 316 https://doi.org/10.1016/j.snb.2020.128097	journal	August 2020
Polariton-Assisted Cooperativity of Molecules in Microcavities Monitored by Two-Dimensional Infrared Spectroscopy Zhang, Zhedong; Wang, Kai; Yi, Zhenhuan The Journal of Physical Chemistry Letters, Vol. 10, Issue 15 https://doi.org/10.1021/acs.jpclett.9b00979	journal	July 2019
Controlling photons using electromagnetically induced transparency Lukin, M. D.; Imamoğlu, A. Nature, Vol. 413, Issue 6853 https://doi.org/10.1038/35095000	journal	September 2001
Real-time observation of valence electron motion Goulielmakis, Eleftherios; Loh, Zhi-Heng; Wirth, Adrian Nature, Vol. 466, Issue 7307 https://doi.org/10.1038/nature09212	journal	August 2010
Attosecond control of electrons emitted from a nanoscale metal tip Krüger, Michael; Schenk, Markus; Hommelhoff, Peter Nature, Vol. 475, Issue 7354 https://doi.org/10.1038/nature10196	journal	July 2011
Reconstruction and control of a time-dependent two-electron wave packet Ott, Christian; Kaldun, Andreas; Argenti, Luca Nature, Vol. 516, Issue 7531 https://doi.org/10.1038/nature14026	journal	December 2014
Spectral phase measurement of a Fano resonance using tunable attosecond pulses Kotur, M.; Guénot, D.; Jiménez-Galán, Á Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms10566	journal	February 2016
Attosecond molecular dynamics: fact or fiction? Lépine, Franck; Ivanov, Misha Y.; Vrakking, Marc J. J. Nature Photonics, Vol. 8, Issue 3 https://doi.org/10.1038/nphoton.2014.25	journal	February 2014
Attosecond imaging of molecular electronic wavepackets Haessler, S.; Caillat, J.; Boutu, W. Nature Physics, Vol. 6, Issue 3 https://doi.org/10.1038/nphys1511	journal	January 2010
Double ionization probed on the attosecond timescale Månsson, Erik P.; Guénot, Diego; Arnold, Cord L. Nature Physics, Vol. 10, Issue 3 https://doi.org/10.1038/nphys2880	journal	January 2014
Attosecond correlation dynamics Ossiander, M.; Siegrist, F.; Shirvanyan, V. Nature Physics, Vol. 13, Issue 3 https://doi.org/10.1038/nphys3941	journal	November 2016
Sub-cycle Oscillations in Virtual States Brought to Light Chini, Michael; Wang, Xiaowei; Cheng, Yan Scientific Reports, Vol. 3, Issue 1 https://doi.org/10.1038/srep01105	journal	January 2013
Molecular polaritons for controlling chemistry with quantum optics Herrera, Felipe; Owrutsky, Jeffrey The Journal of Chemical Physics, Vol. 152, Issue 10 https://doi.org/10.1063/1.5136320	journal	March 2020
Optically Forbidden Excitations of 3 s Electron of Argon by Fast Electron Impact Lin-Fan, Zhu; Hua-Dong, Cheng; Xiao-Jing, Liu Chinese Physics Letters, Vol. 20, Issue 10 https://doi.org/10.1088/0256-307X/20/10/318	journal	September 2003
Angular-distribution parameters and R -matrix calculations of Ar resonances Berrah, N.; Langer, B.; Bozek, J. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 29, Issue 22 https://doi.org/10.1088/0953-4075/29/22/013	journal	November 1996
K-matrix method with B-splines: σ_nell, β_nand resonances in He photoionization belowN= 4 threshold Argenti, Luca; Moccia, Roberto Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 39, Issue 12 https://doi.org/10.1088/0953-4075/39/12/012	journal	May 2006
Probing time-ordering in two-photon double ionization of helium on the attosecond time scale Pazourek, Renate; Nagele, Stefan; Burgdörfer, Joachim Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 48, Issue 6 https://doi.org/10.1088/0953-4075/48/6/061002	journal	March 2015
Doubly resonant photoionization of He below theN= 2 ionization threshold Mihelič, Andrej; Žitnik, Matjaž; Hrast, Mateja Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 50, Issue 24 https://doi.org/10.1088/1361-6455/aa9621	journal	November 2017
Effects of Configuration Interaction on Intensities and Phase Shifts Fano, U. Physical Review, Vol. 124, Issue 6 https://doi.org/10.1103/PhysRev.124.1866	journal	December 1961
Line Profiles in the Far-uv Absorption Spectra of the Rare Gases Fano, U.; Cooper, J. W. Physical Review, Vol. 137, Issue 5A https://doi.org/10.1103/PhysRev.137.A1364	journal	March 1965
Space Quantization in a Gyrating Magnetic Field Rabi, I. I. Physical Review, Vol. 51, Issue 8 https://doi.org/10.1103/PhysRev.51.652	journal	April 1937
On the Derivation of the Dispersion Formula for Nuclear Reactions Siegert, A. J. F. Physical Review, Vol. 56, Issue 8 https://doi.org/10.1103/PhysRev.56.750	journal	October 1939
Excitation-energy transfer under strong laser drive Wang, Xuanhua; Zhang, Zhedong; Wang, Jin Physical Review A, Vol. 103, Issue 1 https://doi.org/10.1103/PhysRevA.103.013516	journal	January 2021
Multipolariton control in attosecond transient absorption of autoionizing states Yanez-Pagans, S.; Cariker, C.; Shaikh, M. Physical Review A, Vol. 105, Issue 6 https://doi.org/10.1103/PhysRevA.105.063107	journal	June 2022
Ultrafast dynamics of the Rydberg states of CO2 : Autoionization and dissociation lifetimes Biswas, D.; Wood, J. K.; Shalaby, I. Physical Review A, Vol. 110, Issue 4 https://doi.org/10.1103/PhysRevA.110.043106	journal	October 2024
Siegert-state expansion for nonstationary systems: Coupled equations in the one-channel case Tolstikhin, Oleg I. Physical Review A, Vol. 73, Issue 6 https://doi.org/10.1103/PhysRevA.73.062705	journal	June 2006
Theory of ultrafast autoionization dynamics of Fano resonances Chu, W. -C.; Lin, C. D. Physical Review A, Vol. 82, Issue 5 https://doi.org/10.1103/PhysRevA.82.053415	journal	November 2010
Transient absorption and reshaping of ultrafast XUV light by laser-dressed helium Gaarde, Mette B.; Buth, Christian; Tate, Jennifer L. Physical Review A, Vol. 83, Issue 1 https://doi.org/10.1103/PhysRevA.83.013419	journal	January 2011
Transmission of an isolated attosecond pulse in a strong-field dressed atom Pfeiffer, Adrian N.; Leone, Stephen R. Physical Review A, Vol. 85, Issue 5 https://doi.org/10.1103/PhysRevA.85.053422	journal	May 2012
Multiconfigurational Hartree-Fock close-coupling ansatz: Application to the argon photoionization cross section and delays Carette, T.; Dahlström, J. M.; Argenti, L. Physical Review A, Vol. 87, Issue 2 https://doi.org/10.1103/PhysRevA.87.023420	journal	February 2013
Photoionization of helium by attosecond pulses: Extraction of spectra from correlated wave functions Argenti, Luca; Pazourek, Renate; Feist, Johannes Physical Review A, Vol. 87, Issue 5 https://doi.org/10.1103/PhysRevA.87.053405	journal	May 2013
Time-domain perspective on Autler-Townes splitting in attosecond transient absorption of laser-dressed helium atoms Wu, Mengxi; Chen, Shaohao; Gaarde, Mette B. Physical Review A, Vol. 88, Issue 4 https://doi.org/10.1103/PhysRevA.88.043416	journal	October 2013
Attosecond XUV absorption spectroscopy of doubly excited states in helium atoms dressed by a time-delayed femtosecond infrared laser Yang, Z. Q.; Ye, D. F.; Ding, Thomas Physical Review A, Vol. 91, Issue 1 https://doi.org/10.1103/PhysRevA.91.013414	journal	January 2015
Dressing effects in the attosecond transient absorption spectra of doubly excited states in helium Argenti, L.; Jiménez-Galán, Á.; Marante, C. Physical Review A, Vol. 91, Issue 6 https://doi.org/10.1103/PhysRevA.91.061403	journal	June 2015
Photoelectron angular distributions in bichromatic atomic ionization induced by circularly polarized VUV femtosecond pulses Douguet, Nicolas; Grum-Grzhimailo, Alexei N.; Gryzlova, Elena V. Physical Review A, Vol. 93, Issue 3 https://doi.org/10.1103/PhysRevA.93.033402	journal	March 2016
Physically feasible three-level transitionless quantum driving with multiple Schrödinger dynamics Song, Xue-Ke; Ai, Qing; Qiu, Jing Physical Review A, Vol. 93, Issue 5 https://doi.org/10.1103/PhysRevA.93.052324	journal	May 2016
Attosecond transient-absorption dynamics of xenon core-excited states in a strong driving field Kobayashi, Yuki; Timmers, Henry; Sabbar, Mazyar Physical Review A, Vol. 95, Issue 3 https://doi.org/10.1103/PhysRevA.95.031401	journal	March 2017
Attosecond Time-Resolved Autoionization of Argon Wang, He; Chini, Michael; Chen, Shouyuan Physical Review Letters, Vol. 105, Issue 14 https://doi.org/10.1103/PhysRevLett.105.143002	journal	October 2010
Subcycle ac Stark Shift of Helium Excited States Probed with Isolated Attosecond Pulses Chini, Michael; Zhao, Baozhen; Wang, He Physical Review Letters, Vol. 109, Issue 7 https://doi.org/10.1103/PhysRevLett.109.073601	journal	August 2012
Attosecond-Recollision-Controlled Selective Fragmentation of Polyatomic Molecules Xie, Xinhua; Doblhoff-Dier, Katharina; Roither, Stefan Physical Review Letters, Vol. 109, Issue 24 https://doi.org/10.1103/PhysRevLett.109.243001	journal	December 2012
Modulation of Attosecond Beating in Resonant Two-Photon Ionization Jiménez-Galán, Álvaro; Argenti, Luca; Martín, Fernando Physical Review Letters, Vol. 113, Issue 26 https://doi.org/10.1103/PhysRevLett.113.263001	journal	December 2014
Attosecond Delays in Molecular Photoionization Huppert, Martin; Jordan, Inga; Baykusheva, Denitsa Physical Review Letters, Vol. 117, Issue 9 https://doi.org/10.1103/PhysRevLett.117.093001	journal	August 2016
Autoionizing Polaritons in Attosecond Atomic Ionization Harkema, N.; Cariker, C.; Lindroth, E. Physical Review Letters, Vol. 127, Issue 2 https://doi.org/10.1103/PhysRevLett.127.023202	journal	July 2021
Laser-Intensity Effect on the Configuration Interaction in Multiphoton Ionization and Autoionization Kim, Young Soon; Lambropoulos, P. Physical Review Letters, Vol. 49, Issue 23 https://doi.org/10.1103/PhysRevLett.49.1698	journal	December 1982
Cavity-Induced Modifications of Molecular Structure in the Strong-Coupling Regime Galego, Javier; Garcia-Vidal, Francisco J.; Feist, Johannes Physical Review X, Vol. 5, Issue 4 https://doi.org/10.1103/PhysRevX.5.041022	journal	November 2015
Exponential Improvement in Photon Storage Fidelities Using Subradiance and “Selective Radiance” in Atomic Arrays Asenjo-Garcia, A.; Moreno-Cardoner, M.; Albrecht, A. Physical Review X, Vol. 7, Issue 3 https://doi.org/10.1103/PhysRevX.7.031024	journal	August 2017
Electromagnetically induced transparency: Optics in coherent media Fleischhauer, Michael; Imamoglu, Atac; Marangos, Jonathan P. Reviews of Modern Physics, Vol. 77, Issue 2 https://doi.org/10.1103/RevModPhys.77.633	journal	July 2005
Comparison of quantum and semiclassical radiation theories with application to the beam maser Jaynes, E. T.; Cummings, F. W. Proceedings of the IEEE, Vol. 51, Issue 1 https://doi.org/10.1109/PROC.1963.1664	journal	January 1963
Comment on "Coherent Control of Retinal Isomerization in Bacteriorhodopsin" Joffre, Manuel Science, Vol. 317, Issue 5837 https://doi.org/10.1126/science.1137011	journal	July 2007
Lorentz Meets Fano in Spectral Line Shapes: A Universal Phase and Its Laser Control Ott, C.; Kaldun, A.; Raith, P. Science, Vol. 340, Issue 6133 https://doi.org/10.1126/science.1234407	journal	May 2013
Controlling Atomic Line Shapes Lin, C. D.; Chu, W. -C. Science, Vol. 340, Issue 6133 https://doi.org/10.1126/science.1238396	journal	May 2013
Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron Gruson, V.; Barreau, L.; Jiménez-Galan, Á. Science, Vol. 354, Issue 6313 https://doi.org/10.1126/science.aah5188	journal	November 2016
Krylov Subspace Methods on Supercomputers Saad, Youcef SIAM Journal on Scientific and Statistical Computing, Vol. 10, Issue 6 https://doi.org/10.1137/0910073	journal	November 1989
Attosecond chirp effect on the transient absorption spectrum of laser-dressed helium atom Zhao, Haiwen; Liu, Candong; Zheng, Yinghui Optics Express, Vol. 25, Issue 7 https://doi.org/10.1364/OE.25.007707	journal	March 2017
Ultrafast magnetic scattering on ferrimagnets enabled by a bright Yb-based soft x-ray source Fan, G.; Légaré, K.; Cardin, V. Optica, Vol. 9, Issue 4 https://doi.org/10.1364/OPTICA.443440	journal	April 2022

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