Exchange bias and interface-related effects in two-dimensional van der Waals magnetic heterostructures: Open questions and perspectives

Phan, Manh-Huong; Kalappattil, Vijaysankar; Jimenez, Valery Ortiz; Thi Hai Pham, Yen; Mudiyanselage, Nivarthana W.Y.A.Y.; Detellem, Derick; Hung, Chang-Ming; Chanda, Amit; Eggers, Tatiana

doi:10.1016/j.jallcom.2022.168375

Exchange bias and interface-related effects in two-dimensional van der Waals magnetic heterostructures: Open questions and perspectives

Journal Article · Fri Dec 09 00:00:00 EST 2022 · Journal of Alloys and Compounds

DOI:https://doi.org/10.1016/j.jallcom.2022.168375· OSTI ID:2419219

^[1]; Kalappattil, Vijaysankar ^[2]; Jimenez, Valery Ortiz ^[2]; Thi Hai Pham, Yen ^[2]; Mudiyanselage, Nivarthana W.Y.A.Y. ^[2]; Detellem, Derick ^[2]; Hung, Chang-Ming ^[2]; Chanda, Amit ^[2]; Eggers, Tatiana ^[2]

Univ. of South Florida, Tampa, FL (United States); OSTI
Univ. of South Florida, Tampa, FL (United States)

The exchange bias (EB) effect is known as a fundamentally and technologically important magnetic property of a magnetic bilayer film. It is manifested as a horizontal shift in a magnetic hysteresis loop of a film subject to cooling in the presence of a magnetic field. The EB effect in van der Waals (vdW) heterostructures offers a novel approach for tuning the magnetic properties of the newly discovered single-layer magnets, as well as adds a new impetus to magnetic vdW heterostructures. Indeed, intriguing EB effects have recently been reported in a variety of low-dimensional vdW magnetic systems ranging from a weakly interlayer-coupled vdW magnet (e.g., Fe₃GeTe₂) to a bilayer composed of two different magnetic vdW materials (e.g., Fe₃GeTe₂/CrCl₃, Fe₃GeTe₂/FePS₃, Fe₃GeTe₂/MnPS₃, Fe₃GeTe₂/CrSe, Fe₃GeTe₂/CrOCl, Fe₃GeTe₂/CoPc, Fe₅GeTe₂/FePS₃), to bilayers of two different vdW defective magnets (e.g., VSe₂/MoS₂), or to metallic ferromagnet/vdW defective magnet interfaces (e.g., Fe/MoS₂). Despite their huge potential in spintronic device applications, the physical origins of the observed EB effects have remained elusive to researchers. Here, we present here a critical review of the EB effect and associated phenomena such as magnetic proximity (MP) in various vdW heterostructure systems and propose approaches to addressing some of the emerging fundamental questions.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of South Florida, Tampa, FL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: FG02-07ER46438

OSTI ID:: 2419219

Alternate ID(s):: OSTI ID: 1905181

Journal Information:: Journal of Alloys and Compounds, Journal Name: Journal of Alloys and Compounds Journal Issue: C Vol. 937; ISSN 0925-8388

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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2D magnets
36 MATERIALS SCIENCE
Exchange bias
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Optospintronics
Spin-caloritronics
Spintronics
Valleytronics
Van der Waals heterostructures

Exchange bias and interface-related effects in two-dimensional van der Waals magnetic heterostructures: Open questions and perspectives

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