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Semiclassical theory of bipolaronic superconductivity in a bond-modulated electron-phonon model

Journal Article · · Physical Review. B
 [1];  [2];  [3]
  1. Stanford University, CA (United States); SLAC
  2. Stanford University, CA (United States)
  3. Stanford University, CA (United States); University of California, San Diego, La Jolla, CA (United States)

We analyze the transition temperature Tc of bipolaronic superconductivity in a bond Su-Schrieffer-Heeger (bond-SSH) model—also known as a bond Peierls model—where the electron hoppings are modulated by bond phonons. Using a semiclassical instanton approximation justifiable in the adiabatic limit of slow phonons, we find that the bipolaron mass is only weakly enhanced, in contrast to the typical large mass enhancement found in standard (Holstein) electron-phonon models. Specifically, in the strong coupling limit, the bipolarons can freely slide within a degenerate manifold rather than become self-trapped. A gas of these bipolarons can undergo a superfluid transition at a critical temperature for which we obtain an upper bound. We find that this bound is exponentially larger than that in the Holstein model. In conclusion, our study provides an analytical understanding of the mechanism behind the high-Tc bipolaronic superconductivity numerically observed in [Phys. Rev. X 13, 011010 (2023)].

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); Gordon and Betty Moore Foundation’s EPiQS Initiative
Grant/Contract Number:
AC02-76SF00515
OSTI ID:
2404898
Alternate ID(s):
OSTI ID: 2474313
Journal Information:
Physical Review. B, Journal Name: Physical Review. B Journal Issue: 22 Vol. 109; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (39)

Squeezed bipolaronic states and high temperature superconductivity in BaLaCuO systems journal November 1987
Eliashberg theory of phonon-mediated superconductivity — When it is valid and how it breaks down journal June 2020
Condensed Matter Field Theory book August 2010
A bound on the superconducting transition temperature journal November 2018
Heuristic bounds on superconductivity and how to exceed them journal August 2022
High-temperature superconductivity journal May 2021
Possibility of insulator to superconductor phase transition journal January 1979
Quantum Field Theory and Critical Phenomena book April 2021
Fractons from polarons journal December 2020
Bond-Peierls polaron: Moderate mass enhancement and current-carrying ground state journal October 2021
Bipolaron liquids at strong Peierls electron-phonon couplings journal November 2021
Valence-bond solid to antiferromagnet transition in the two-dimensional Su-Schrieffer-Heeger model by Langevin dynamics journal February 2022
Phase diagram of the Su-Schrieffer-Heeger-Hubbard model on a square lattice journal August 2022
Robustness of antiferromagnetism in the Su-Schrieffer-Heeger Hubbard model journal August 2022
Comparative determinant quantum Monte Carlo study of the acoustic and optical variants of the Su-Schrieffer-Heeger model journal October 2023
Comparative study of the superconductivity in the Holstein and optical Su-Schrieffer-Heeger models journal November 2023
Attractive Su-Schrieffer-Heeger-Hubbard model on a square lattice away from half-filling journal October 2023
Bipolaronic superconductivity out of a Coulomb gas journal December 2023
Charge bond order and s -wave superconductivity in the kagome lattice with electron-phonon coupling and electron-electron interaction journal February 2024
Phases and exotic phase transitions of a two-dimensional Su-Schrieffer-Heeger model journal May 2024
Dilute Bose gas in two dimensions journal April 1988
Multiparticle ring exchange in the Wigner glass and its possible relevance to strongly interacting two-dimensional electron systems in the presence of disorder journal November 2001
Two bounds on the maximum phonon-mediated superconducting transition temperature journal September 2006
Generalized inverse participation ratio as a possible measure of localization for interacting systems journal May 2011
Breakdown of the Migdal-Eliashberg theory: A determinant quantum Monte Carlo study journal April 2018
Pseudogap crossover in the electron-phonon system journal May 2019
Critical Temperature of Interacting Bose Gases in Two and Three Dimensions journal April 2008
Consistency of the Adiabatic Theorem journal June 2009
Light Bipolarons Stabilized by Peierls Electron-Phonon Coupling journal December 2018
Strong Coupling Limit of the Holstein-Hubbard Model journal October 2020
Quantum Monte Carlo Simulations of the 2D Su-Schrieffer-Heeger Model journal January 2021
Antiferromagnetism Induced by Bond Su-Schrieffer-Heeger Electron-Phonon Coupling: A Quantum Monte Carlo Study journal December 2021
Resonating Valence Bond States in an Electron-Phonon System journal May 2023
Emergent Inflation of the Efimov Spectrum under Three-Body Spin-Exchange Interactions journal March 2024
Mobile Bipolaron journal April 2000
Critical Point of a Weakly Interacting Two-Dimensional Bose Gas journal December 2001
Bipolaronic High-Temperature Superconductivity journal January 2023
Breakdown of the Migdal-Eliashberg theory in the strong-coupling adiabatic regime journal October 2001
Optim: A mathematical optimization package for Julia journal April 2018