Relaxing Wrinkles in Jammed Interfacial Assemblies

Xie, Ganhua; Zhu, Shipei; Kim, Paul Y.; Jiang, Shubao; Yi, Qinpiao; Li, Pei; Chu, Zonglin; Helms, Brett A.; Russell, Thomas P.

doi:10.1002/anie.202307713

Relaxing Wrinkles in Jammed Interfacial Assemblies

Journal Article · Fri Jul 14 04:00:00 EDT 2023 · Angewandte Chemie (International Edition)

DOI:https://doi.org/10.1002/anie.202307713· OSTI ID:2349269

Xie, Ganhua ^[1]; Zhu, Shipei ^[2]; Kim, Paul Y. ^[2]; Jiang, Shubao ^[3]; Yi, Qinpiao ^[3]; Li, Pei ^[4]; Chu, Zonglin ^[3]; Helms, Brett A. ^[5]; ^[6]

Hunan Univ., Changsha (China). Key Lab. for Chemo/Bio-Sensing and Chemometrics; Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Hunan Univ., Changsha (China). Key Lab. for Chemo/Bio-Sensing and Chemometrics
Hunan Univ., Changsha (China)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Molecular Foundry
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Univ. of Massachusetts, Amherst, MA (United States); Tohoku Univ., Sendai (Japan). WPI-Advanced Inst. for Materials Research

Dynamic covalent bonding has emerged as a mean by which stresses in a network can be relaxed. Here, the strength of the bonding of ligands to nanoparticles at the interface between two immiscible liquids affect the same results in jammed assemblies of nanoparticle surfactants. Beyond a critical degree of overcrowding induced by the compression of jammed interfacial assemblies, the bonding of ligands to nanoparticles (NPs) can be broken, resulting in a desorption of the NPs from the interface. This reduces the areal density of nanoparticle surfactants at the interface, allowing the assemblies to relax, not to a fluid state but rather another jammed state. The relaxation of the wrinkles caused by the compression reflects the tendency of these assemblies to eliminate areas of high curvature, favoring a more planar geometry. Importantly, this enabled the generation of giant vesicular and multivesicular structures from these assemblies.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); US Army Research Office (ARO)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 2349269

Journal Information:: Angewandte Chemie (International Edition), Journal Name: Angewandte Chemie (International Edition) Journal Issue: 36 Vol. 62; ISSN 1433-7851

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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