Operational and scaling-up barriers of SOEC and mitigation strategies to boost H2 production- a comprehensive review

Jolaoso, Lateef A.; Bello, Idris T.; Ojelade, Opeyemi A.; Yousuf, Abu; Duan, Chuancheng; Kazempoor, Pejman

doi:10.1016/j.ijhydene.2023.05.077

Operational and scaling-up barriers of SOEC and mitigation strategies to boost H₂ production- a comprehensive review

Journal Article · Fri May 26 00:00:00 EDT 2023 · International Journal of Hydrogen Energy

DOI:https://doi.org/10.1016/j.ijhydene.2023.05.077· OSTI ID:2335866

^[1]; Bello, Idris T. ^[2]; ^[3]; ^[4]; Duan, Chuancheng ^[5]; Kazempoor, Pejman ^[6]

University of Oklahoma, Norman, OK (United States); University of Oklahoma
Hong Kong Polytechnic University, Kowloon (Hong Kong)
Georgia Institute of Technology, Atlanta, GA (United States)
University of Oklahoma, Norman, OK (United States); Shahjalal University of Science and Technology, Sylhet (Bangladesh)
Kansas State University, Manhattan, KS (United States)
University of Oklahoma, Norman, OK (United States)

Solid oxide electrolysis cells (SOECs) proffer a flexible and environmentally friendly solution to reduce CO₂ emissions and/or produce H₂ fuel for various applications. Here, the integration of this technology with renewable energy systems makes them even more promising in realizing a near-perpetual green energy infrastructure in the near future. SOEC technology has achieved stupendous improvement in recent years, and some of the limiting factors to the commercialization of this technology have been explored. It is, therefore, necessary to have a succinct outlook of the different factors that contribute to the recent developments in SOEC technology. The current work presents a comprehensive review of the state-of-the-art SOEC component materials and their degradation mechanisms, SOEC modeling essentials and efficiencies, and the scalability of SOECs. Although SOEC is considered a highly promising technology and sufficient multifaceted research has been done, yet not been widely commercialized. Despite the improvement to mitigate degradation of the SOEC materials, a large share of the degradation concerns sprang from charge transfer reaction at the triple-phase boundaries of the H₂-electrode. Part of which can be improved by microkinetic modeling of these materials supported by their characterization to give insight into their development. Some other directions for the future in advancing this technology toward the commercialization stage are thoroughly addressed.

View Accepted Manuscript (DOE)

Research Organization:: University of Oklahoma, Norman, OK (United States)

Sponsoring Organization:: USDOE; USDOE Office of Fossil Energy and Carbon Management (FECM)

Grant/Contract Number:: FE0032005

OSTI ID:: 2335866

Alternate ID(s):: OSTI ID: 1999322

Journal Information:: International Journal of Hydrogen Energy, Journal Name: International Journal of Hydrogen Energy Journal Issue: 85 Vol. 48; ISSN 0360-3199

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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