Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

High temperature annealing of irradiated nuclear grade graphite

Journal Article · · Journal of Nuclear Materials
Previous work has shown that the material properties of nuclear grade graphite are substantially affected by the atomic and microstructural changes that occur during neutron-irradiation. The parameters that play a role in these changes are irradiation dose, temperature, graphite composition and the initial microstructure of the graphite. Understanding the details of how these material changes occur and exactly what the changes consists of will enable the prediction of the material property changes as a function of these variables. Other work has shown these atomic level and microstructural changes can be healed or annealed out by raising the irradiated graphite above its irradiation temperature. Here in this work, experiments were carried out to investigate how the properties of irradiated graphite recover when heated. By showing property recovery as a function of annealing temperature or energy, insight is provided into the type of damage that occurred during neutron-irradiation. The data presented here shows recovery of thermal diffusivity, coefficient of thermal expansion, Young's modulus and electrical resistivity between annealing temperatures of 500 °C and 2380 °C. Graphite grades NBG-18, IG-110 and PCEA are considered that were both stressed and unstressed during irradiation.
Research Organization:
Idaho National Laboratory (INL), Idaho Falls, ID (United States)
Sponsoring Organization:
58; USDOE; USDOE Office of Energy Efficiency and Renewable Energy (EERE)
Grant/Contract Number:
AC07-05ID14517
OSTI ID:
2332722
Alternate ID(s):
OSTI ID: 1963345
Report Number(s):
INL/JOU--22-68425-Revision-0
Journal Information:
Journal of Nuclear Materials, Journal Name: Journal of Nuclear Materials Journal Issue: - Vol. 579; ISSN 0022-3115
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (35)

The theory of irradiation creep in reactor graphite—The dislocation pinning-unpinning model journal April 1974
The role of porosity in the accommodation of thermal expansion in graphite journal September 1962
Irradiation damage to pile grade graphite at 450° C journal December 1962
Thermal annealing effects on electrical resistivity of reactor grade graphite irradiated with neutrons at 250 °C and 350 °C journal November 1971
The effects of radiation damage on the properties of GraphNOL N3M journal March 1991
Thermal conductivity degradation of graphites due to nuetron irradiation at low temperature journal September 1995
A study of the annealing behavior of neutron irradiated graphite journal January 2011
Proton irradiation-induced creep of ultra-fine grain graphite journal October 2014
Neutron irradiation induced microstructural changes in NBG-18 and IG-110 nuclear graphites journal May 2015
Property changes of G347A graphite due to neutron irradiation journal November 2016
Thermal annealing of nuclear graphite during in-situ electron irradiation journal May 2017
Historical experiment to measure irradiation-induced creep of graphite journal November 2018
Development of mesopores in superfine grain graphite neutron-irradiated at high fluence journal January 2019
Formation of carbon nanostructures in nuclear graphite under high-temperature in situ electron-irradiation journal March 2019
Experimental evidence for ‘buckle, ruck and tuck’ in neutron irradiated graphite journal April 2020
Vacancy-driven variations in the phonon density of states of fast neutron irradiated nuclear graphite journal October 2020
Fullerene-like defects in high-temperature neutron-irradiated nuclear graphite journal September 2020
A macro-scale ruck and tuck mechanism for deformation in ion-irradiated polycrystalline graphite journal March 2021
Prismatic edge dislocations in graphite journal March 2022
Constitutive material model for the prediction of stresses in irradiated anisotropic graphite components journal October 2008
In situ transmission electron microscopy of electron-beam induced damage process in nuclear grade graphite journal May 2011
Buckle, ruck and tuck: A proposed new model for the response of graphite to neutron irradiation journal June 2011
Comparison of irradiation behaviour of HTR graphite grades journal August 2017
Microstructural changes in nuclear graphite induced by thermal annealing journal December 2022
Wigner defects bridge the graphite gap journal April 2003
Damage process in electron-irradiated graphite studied by transmission electron microscopy. I. High-resolution observation of highly graphitized carbon fibre journal September 1997
Dimensional change, irradiation creep and thermal/mechanical property changes in nuclear graphite journal April 2016
Radiation defects in graphite journal November 2007
Modelling of dimensional changes in irradiated nuclear graphites journal October 2000
Radiation damage of graphite - degradation of material parameters and defect structures journal January 1996
Transmission Electron Microscopy Study of Graphite under in situ Ion Irradiation journal July 2012
Local structural order in electron-irradiated graphite studied by high-resolution high-voltage electron microscopy journal January 1999
Ripplocations in layered materials: Sublinear scaling and basal climb journal May 2021
Dimensional changes in highly oriented pyrolytic graphite due to electron-irradiation journal July 1994
Ripplocations: A Progress Report journal May 2020

Similar Records

HIGH TEMPERATURE ANNEALING OF IRRADIATED NUCLEAR GRADE GRAPHITE
Conference · Mon Oct 08 00:00:00 EDT 2018 · OSTI ID:1484477

The Innograph irradiations; HTR graphite material properties from 0 to 25 DPA - 18541
Conference · Mon Nov 14 23:00:00 EST 2016 · OSTI ID:23032681

Initial Comparison of Baseline Physical and Mechanical Properties for the VHTR Candidate Graphite Grades
Technical Report · Mon Sep 01 00:00:00 EDT 2014 · OSTI ID:1168626