Silica‐Derived Nanostructured Electrode Materials for ORR, OER, HER, CO 2 RR Electrocatalysis, and Energy Storage Applications: A Review**

Onajah, Sammy; Sarkar, Rajib; Islam, Md. Shafiul; Lalley, Marja; Khan, Kishwar; Demir, Muslum; Abdelhamid, Hani Nasser; Farghaly, Ahmed A.

doi:10.1002/tcr.202300234

Title: Silica‐Derived Nanostructured Electrode Materials for ORR, OER, HER, CO ₂ RR Electrocatalysis, and Energy Storage Applications: A Review**

Journal Article · Tue Mar 26 00:00:00 EDT 2024 · Chemical Record

DOI:https://doi.org/10.1002/tcr.202300234· OSTI ID:2328652

Onajah, Sammy ^[1]; Sarkar, Rajib ^[2]; Islam, Md. Shafiul ^[3]; Lalley, Marja ^[4]; Khan, Kishwar ^[5]; Demir, Muslum ^[6]; Abdelhamid, Hani Nasser ^[7];

^[8]

Chemical Sciences and Engineering Division Argonne National Laboratory Lemont Illinois 60439 United States, Pritzker School of Molecular Engineering The University of Chicago Chicago Illinois 60637 United States
Department of Chemistry Virginia Commonwealth University Richmond Virginia 23284-2006 United States
Chemical Sciences and Engineering Division Argonne National Laboratory Lemont Illinois 60439 United States
Department of Chemistry University of Chicago Chicago Illinois 60637 United States
Department of Chemistry City University of Hong Kong Hong Kong 999077 China
Department of Chemical Engineering Bogazici University 34342 Istanbul Turkey, TUBITAK Marmara Research Center Material Institute Gebze 41470 Turkey
Advanced Multifunctional Materials Laboratory Department of Chemistry Assiut University Assiut 71516 Egypt, Egyptian Russian University Badr City Cairo 11829 Egypt
Chemical Sciences and Engineering Division Argonne National Laboratory Lemont Illinois 60439 United States, Pritzker School of Molecular Engineering The University of Chicago Chicago Illinois 60637 United States, Chemistry Department Faculty of Science Assiut University Assiut 71516 Egypt

Abstract Silica‐derived nanostructured catalysts (SDNCs) are a class of materials synthesized using nanocasting and templating techniques, which involve the sacrificial removal of a silica template to generate highly porous nanostructured materials. The surface of these nanostructures is functionalized with a variety of electrocatalytically active metal and non‐metal atoms. SDNCs have attracted considerable attention due to their unique physicochemical properties, tunable electronic configuration, and microstructure. These properties make them highly efficient catalysts and promising electrode materials for next generation electrocatalysis, energy conversion, and energy storage technologies. The continued development of SDNCs is likely to lead to new and improved electrocatalysts and electrode materials. This review article provides a comprehensive overview of the recent advances in the development of SDNCs for electrocatalysis and energy storage applications. It analyzes 337,061 research articles published in the Web of Science (WoS) database up to December 2022 using the keywords “silica”, “electrocatalysts”, “ORR”, “OER”, “HER”, “HOR”, “CO ₂ RR”, “batteries”, and “supercapacitors”. The review discusses the application of SDNCs for oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), carbon dioxide reduction reaction (CO ₂ RR), supercapacitors, lithium‐ion batteries, and thermal energy storage applications. It concludes by discussing the advantages and limitations of SDNCs for energy applications.

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Sponsoring Organization:: USDOE

OSTI ID:: 2328652

Alternate ID(s):: OSTI ID: 2336856

Journal Information:: Chemical Record, Journal Name: Chemical Record Vol. 24 Journal Issue: 4; ISSN 1527-8999

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: United States

Language:: English

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