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Title: Process Modeling of Aerosol‐Cloud Interaction in Summertime Precipitating Shallow Cumulus Over the Western North Atlantic

Journal Article · · Journal of Geophysical Research. Atmospheres
DOI:https://doi.org/10.1029/2023JD039489· OSTI ID:2328649
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  1. Pacific Northwest National Laboratory Richland WA USA
  2. Institut für Physik der Atmosphäre Deutsches Zentrum für Luft‐ und Raumfahrt (DLR) and Institute for Physics of the Atmosphere Johannes Gutenberg‐University Mainz Mainz Germany
  3. NASA Langley Research Center Hampton VA USA, Analytical Mechanics Associates Hampton VA USA
  4. NASA Langley Research Center Hampton VA USA
  5. Department of Chemical and Environmental Engineering University of Arizona Tucson AZ USA
  6. Department of Hydrology and Atmospheric Sciences University of Arizona Tucson AZ USA
  7. University of Arizona James C. Wyant College of Optical Sciences Tucson AZ USA
  8. Department of Chemical and Environmental Engineering University of Arizona Tucson AZ USA, Department of Hydrology and Atmospheric Sciences University of Arizona Tucson AZ USA
  9. NASA Langley Research Center Hampton VA USA, Coherent Applications, Inc. Hampton VA USA
  10. NASA Langley Research Center Hampton VA USA, NASA Postdoctoral Program NASA Langley Research Center Hampton VA USA
  11. NASA Goddard Institute for Space Studies New York NY USA

Abstract Process modeling of Aerosol‐cloud interaction (ACI) is essential to bridging gaps between observational analysis and climate modeling of aerosol effects in the Earth system and eventually reducing climate projection uncertainties. In this study, we examine ACI in summertime precipitating shallow cumuli observed during the Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE). Aerosols and precipitating shallow cumuli were extensively observed with in‐situ and remote‐sensing instruments during two research flight cases on 02 June and 07 June, respectively, during the ACTIVATE summer 2021 deployment phase. We perform observational analysis and large‐eddy simulation (LES) of aerosol effect on precipitating cumulus in these two cases. Given the measured aerosol size distributions and meteorological conditions, LES is able to reproduce the observed cloud properties by aircraft such as liquid water content (LWC), cloud droplet number concentration ( N c ) and effective radius r eff . However, it produces smaller liquid water path (LWP) and larger N c compared to the satellite retrievals. Both 02 and 07 June cases are over warm waters of the Gulf Stream and have a cloud top height over 3 km, but the 07 June case is more polluted and has larger LWC. We find that the N a ‐induced LWP adjustment is dominated by precipitation feedback for the 2 June precipitating case and there is no clear entrainment feedback in both cases. An increase of cloud fraction due to a decrease of aerosol number concentration is also shown in the simulations for the 02 June case.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE; National Aeronautics and Space Administration (NASA)
Grant/Contract Number:
AC05-76RL01830
OSTI ID:
2328649
Alternate ID(s):
OSTI ID: 2336733; OSTI ID: 2337561
Report Number(s):
PNNL-SA-186592; e2023JD039489
Journal Information:
Journal of Geophysical Research. Atmospheres, Journal Name: Journal of Geophysical Research. Atmospheres Vol. 129 Journal Issue: 7; ISSN 2169-897X
Publisher:
American Geophysical Union (AGU)Copyright Statement
Country of Publication:
United States
Language:
English

References (26)

Simulating Aerosol Lifecycle Impacts on the Subtropical Stratocumulus‐to‐Cumulus Transition Using Large‐Eddy Simulations journal October 2022
On the precipitation susceptibility of clouds to aerosol perturbations journal January 2009
High Climate Sensitivity in the Community Earth System Model Version 2 (CESM2) journal July 2019
Bounding global aerosol radiative forcing of climate change journal November 2019
Rain in Shallow Cumulus Over the Ocean: The RICO Campaign journal December 2007
Assessment of MODIS cloud effective radius and optical thickness retrievals over the Southeast Pacific with VOCALS-REx in situ measurements: MODIS VALIDATION DURING VOCALS-REx journal December 2011
Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability journal February 2016
Dataset for paper "Process Modeling of Aerosol-cloud Interaction in Summertime Precipitating Shallow Cumulus over the Western North Atlantic" dataset January 2023
The impact of humidity above stratiform clouds on indirect aerosol climate forcing journal December 2004
Effect of Aerosol on the Susceptibility and Efficiency of Precipitation in Warm Trade Cumulus Clouds journal November 2010
Aerosols, Cloud Microphysics, and Fractional Cloudiness journal September 1989
Modeling Mesoscale Cellular Structures and Drizzle in Marine Stratocumulus. Part I: Impact of Drizzle on the Formation and Evolution of Open Cells journal November 2009
Aerosols enhance cloud lifetime and brightness along the stratus-to-cumulus transition journal July 2020
Open-path airborne tunable diode laser hygrometer
  • Diskin, Glenn S.; Podolske, James R.; Sachse, Glen W.
  • International Symposium on Optical Science and Technology, SPIE Proceedings https://doi.org/10.1117/12.453736
conference September 2002
ERA5 hourly data on single levels from 1940 to present dataset March 2024
Aerosol-cloud-climate cooling overestimated by ship-track data journal January 2021
Polarimeter + Lidar–Derived Aerosol Particle Number Concentration journal May 2022
The 2D-S (Stereo) Probe: Design and Preliminary Tests of a New Airborne, High-Speed, High-Resolution Particle Imaging Probe journal November 2006
Stratocumulus to Cumulus Transition by Drizzle: STRATOCUMULUS TO CUMULUS BY DRIZZLE journal October 2017
A single parameter representation of hygroscopic growth and cloud condensation nucleus activity journal January 2007
Substantial Cloud Brightening From Shipping in Subtropical Low Clouds journal March 2020
On the Factors Modulating the Stratocumulus to Cumulus Transitions journal September 2011
Improving our fundamental understanding of the role of aerosol−cloud interactions in the climate system journal May 2016
Impact of Cloud Microphysics on the Development of Trailing Stratiform Precipitation in a Simulated Squall Line: Comparison of One- and Two-Moment Schemes journal March 2009
Evaluation of Scalar Advection Schemes in the Advanced Research WRF Model Using Large-Eddy Simulations of Aerosol–Cloud Interactions journal August 2009
RACORO continental boundary layer cloud investigations: 2. Large-eddy simulations of cumulus clouds and evaluation with in situ and ground-based observations: LES OF RACORO BOUNDARY LAYER CUMULI journal June 2015