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Photochemical modeling of the impact of fuels and vehicles on urban ozone using auto/oil program data

Journal Article · · Environmental Science and Technology
DOI:https://doi.org/10.1021/es950175m· OSTI ID:232453
 [1]; ; ;  [2];  [3]
  1. General Motors Research and Development Center, Warren, MI (United States)
  2. Systems Applications International, San Rafael, CA (United States)
  3. Mobil Research and Development Corporation. Paulsboro, NJ (United States)

An extensive set of emission tests has been conducted in the Auto/Oil Air Quality Improvement Research Program on different fuel/vehicle systems. These emission tests have been used to model the impact of fuel/vehicle changes on ozone formation in Los Angeles, Dallas-Fort Worth, and New York in 1995 and 2005/2010. Light-duty vehicles are estimated to contribute 28-37% of the peak ozone in 1980/1985, decreasing to 7-18% in 1995, and further decreasing to 5-9% in 2005/2010. Gasoline changes that show promise in reducing the contribution of light-duty vehicles to ozone formation are reductions in olefin content, 90% distillation temperature, sulfur content, and vapor pressure. Results for a methanol/gasoline blend (M85) used in prototype flexible/variable fuel vehicles depend on the assumptions used to project future M85 emissions. A research test gasoline produced less ozone than the M85 cases in Los Angeles and New York and either more or less ozone than M85 in Dallas-Fort Worth, depending on the assumptions. Sensitivity tests for Los Angeles addressed uncertainties in the overall magnitude of emissions from light-duty vehicles, in the biogenic inventory, and in the representation of the atmospheric chemistry. 51 refs., 7 figs., 11 tabs.

OSTI ID:
232453
Journal Information:
Environmental Science and Technology, Journal Name: Environmental Science and Technology Journal Issue: 3 Vol. 30; ISSN ESTHAG; ISSN 0013-936X
Country of Publication:
United States
Language:
English

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