Confinement of 1D Chain and 2D Layered CuI Modules in K-INA-R Frameworks via Coordination Assembly: Structure Regulation and Semiconductivity Tuning

Wu, Zhao-Feng; Wang, Chuanzhe; Liu, Xingwu; Tan, Kui; Fu, Zhihua; Teat, Simon J.; Li, Zi-Wei; Hei, Xiuze; Huang, Xiao-Ying; Xu, Gang; Li, Jing

doi:10.1021/jacs.3c05095

Title: Confinement of 1D Chain and 2D Layered CuI Modules in K-INA-R Frameworks via Coordination Assembly: Structure Regulation and Semiconductivity Tuning

Journal Article · Thu Aug 24 00:00:00 EDT 2023 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.3c05095· OSTI ID:2305736

Wu, Zhao-Feng ^[1]; Wang, Chuanzhe ^[2];

^[3];

^[4]; Fu, Zhihua ^[2]; Teat, Simon J. ^[5]; Li, Zi-Wei ^[6]; Hei, Xiuze ^[7];

^[2];

^[7]

Rutgers University, New Brunswick, NJ (United States); Chinese Academy of Sciences, Fujian (China); Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fujian (China)
Chinese Academy of Sciences, Fujian (China)
Synfuels China Technology Co.Ltd., Beijing (China)
University of North Texas, Denton, TX (United States)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Chinese Academy of Sciences, Fujian (China); Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fujian (China)
Rutgers University, New Brunswick, NJ (United States)

Herein, we present a new series of CuI-based hybrid materials with tunable structures and semiconducting properties. Furthermore, the CuI inorganic modules can be tailored into a one-dimensional (1D) chain and two-dimensional (2D) layer and confined/stabilized in coordination frameworks of potassium isonicotinic acid (HINA) and its derivatives (HINA-R, R = OH, NO₂, and COOH). The resulting CuI-based hybrid materials exhibit interesting semiconducting behaviors associated with the dimensionality of the inorganic module; for instance, the structures containing the 2D-CuI module demonstrate significantly enhanced photoconductivity with a maximum increase of five orders of magnitude compared to that of the structures containing the 1D-CuI module. They also represent the first CuI-bearing hybrid chemiresistive gas sensors for NO₂ with boosted sensing performance and sensitivity at multiple orders of magnitude over that of the pristine CuI. Particularly, the sensing ability of CuI-K-INA containing both 1D- and 2D-CuI modules is comparable to those of the best NO₂ chemiresistors reported thus far.

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Research Organization:: Wake Forest University, Winston-Salem, NC (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0019902; AC02-05CH11231

OSTI ID:: 2305736

Journal Information:: Journal of the American Chemical Society, Vol. 145, Issue 35; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Confinement of 1D Chain and 2D Layered CuI Modules in K-INA-R Frameworks via Coordination Assembly: Structure Regulation and Semiconductivity Tuning

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