Inspection of Dry Storage Casks Using PGAA and NAA Techniques

Journal Article · Fri Jul 01 04:00:00 EDT 2016 · Transactions of the American Nuclear Society

OSTI ID:23042574

Brookman, Jason ^[1]; Shayer, Zeev ^[2]

---

1. Idaho National Laboratory (United States)
2. Department of Physics, Colorado School of Mines (United States)

In this effort, an assessment of a chloride detection method is performed for inspecting the surfaces of dry cask storage system (DCSS) canisters, with focus on the implementation of a non-destructive nuclear analysis and methodology. Some DCSS canisters (especially those located in coastal environments) will be exposed to marine environments, which can cause atmospheric stress corrosion cracking (SCC). Chloride deposits on canister surfaces provide the corrosive environment necessary for atmospheric SCC with the residual stresses and materials properties conditions. The most susceptible regions on the canister surface are the weld areas, or where cold work has been performed, and may provide the necessary driving force for crack growth. The heat-affected zones (HAZs) near welds are also potentially susceptible to atmospheric SCC due to sensitization of the material caused by chromium depletion during the welding process. Information collected from the field and from laboratory studies has not been able to rule out the possibility of atmospheric chloride induced stress corrosion cracking (CISCC), although no occurrences of atmospheric SCC in DCSS canisters have been detected to-date. A number of researchers have demonstrated that localized corrosion can take place under such situations on materials commonly used for interim storage containers, including 304SS (Cook et al. 2010; Shirai et al. 2011) and 316SS (Tani et al. 2009). In this summary, the preliminary results of a neutron activation analysis (NAA) and prompt gamma activation analysis (PGAA) are performed using MCNP6, a highly sophisticated, multi-particle Monte Carlo simulation code (with the employment of the high performance computing system at the Idaho National Laboratory), and confirm the feasibility of using PGAA and NAA as an environmental inspection methodology for detection and monitoring of small quantities of chlorine on canister surfaces. The specific signature of gamma rays due reactions of sea salt constituents are documented and summarized in this paper. The environmental constituent for passive oxide film breaching is chlorine, which can cause pitting initiation and incubation time that may lead to cracking in stainless steel. Therefore, an assessment of chloride presence at a canister surface is essential before moving to other nondestructive analysis (NDA) methods for detection of pitting and cracking. Two nonlinear acoustic techniques will also be used in our integrated research project (IRP) research study that proves to be useful in the detection of SCC: nonlinear resonant ultrasound spectroscopy (NRUS), and time revisited elastic nonlinear diagnostic (TREND). These two techniques are complementary to marine atmospheric detection techniques. In this presentation only PGAA and NAA are described in detail. (authors)

• OSTI ID: 23042574
• Journal Information: Transactions of the American Nuclear Society, Journal Name: Transactions of the American Nuclear Society Vol. 115; ISSN 0003-018X
• Country of Publication: United States
• Language: English

Related Subjects

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY
ACOUSTICS
CHLORIDES
CHLORINE
COMPUTERIZED SIMULATION
CRACK PROPAGATION
CRACKING
DRY STORAGE
GAMMA RADIATION
HEAT AFFECTED ZONE
MONTE CARLO METHOD
NEUTRON ACTIVATION ANALYSIS
RADIOACTIVE WASTE STORAGE
RESIDUAL STRESSES
SPECTROSCOPY
SPENT FUEL CASKS
STAINLESS STEEL-316
STRESS CORROSION
WELDED JOINTS